Phosphate adsorption on hydrous ferric oxide (HFO) at different salinities and pHs.


Journal

Chemosphere
ISSN: 1879-1298
Titre abrégé: Chemosphere
Pays: England
ID NLM: 0320657

Informations de publication

Date de publication:
Jun 2019
Historique:
received: 01 10 2018
revised: 07 03 2019
accepted: 11 03 2019
pubmed: 19 3 2019
medline: 11 7 2019
entrez: 19 3 2019
Statut: ppublish

Résumé

Phosphate adsorption on suspended sediments is largely influenced by the variations in salinity and pH such as is the case in estuaries where freshwater mixes with seawater, exhibiting strong physico-chemical gradients. In this research, the influence of salinity and pH on the adsorption of phosphate on hydrous ferric oxides (HFO) was investigated in NaCl solutions. The adsorption isotherm data at different salinities can be well fitted with the Langmuir-Freundlich model. At pH 8.5 the maximum adsorption capacity increases with increasing salinity, from 22.7 mg PO4/g at salinity 0-78.5 mg PO4/g at salinity 35 PSU (Practical Salinity Unit) with the largest increase occurring in the low salinity range (76.8 mg PO4/g at salinity 5 PSU). Phosphate adsorption is also highly pH dependent and the adsorption capacity decreases with increasing pH. The dependence of phosphate adsorption on salinity could be attributed to the inner-sphere complexation. The presence of Na

Identifiants

pubmed: 30884296
pii: S0045-6535(19)30505-3
doi: 10.1016/j.chemosphere.2019.03.068
pii:
doi:

Substances chimiques

Ferric Compounds 0
Phosphates 0
Solutions 0
ferric oxide 1K09F3G675
ferric hydroxide 2UA751211N
Sodium Chloride 451W47IQ8X

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

352-359

Informations de copyright

Copyright © 2019 Elsevier Ltd. All rights reserved.

Auteurs

Hailong Zhang (H)

Service de Biogéochimie et Modélisation du Système Terre, Université Libre de Bruxelles, Campus de la Plaine - CP 208, Boulevard du Triomphe, B-1050 Brussels, Belgium; Laboratory of Analytical, Environmental and Geo-Chemistry, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussels, Belgium. Electronic address: Hailong.Zhang@ulb.ac.be.

Marc Elskens (M)

Laboratory of Analytical, Environmental and Geo-Chemistry, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussels, Belgium.

Guoxing Chen (G)

4MAT, Université libre de Bruxelles, 50 av. F.D. Roosevelt, 1050 Brussels, Belgium.

Lei Chou (L)

Service de Biogéochimie et Modélisation du Système Terre, Université Libre de Bruxelles, Campus de la Plaine - CP 208, Boulevard du Triomphe, B-1050 Brussels, Belgium.

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Classifications MeSH