An ultra-rapid drug screening method for acetaminophen in blood serum based on probe electrospray ionization-tandem mass spectrometry.


Journal

Journal of food and drug analysis
ISSN: 2224-6614
Titre abrégé: J Food Drug Anal
Pays: China (Republic : 1949- )
ID NLM: 101630927

Informations de publication

Date de publication:
07 2019
Historique:
received: 03 09 2018
revised: 30 01 2019
accepted: 01 02 2019
entrez: 21 7 2019
pubmed: 22 7 2019
medline: 8 7 2020
Statut: ppublish

Résumé

Poisoning incidents caused by drugs, accidental ingestion of poisons, attempted suicide, homicide, and exposure to toxic compounds occur frequently every year across the globe. This raises the need to rapidly identify toxic agents in poisoned patients in a clinical emergency setting. In addition, determining drug/poison concentration is undoubtedly necessary to arrive at a toxicological treatment plan. The purpose of this study was to develop an ultra-rapid drug screening method for the clinical treatment of poisoning. Probe electrospray ionization (PESI), one of the ambient ionization techniques, is able to detect compounds from various biological materials almost directly. We applied the PESI technique to the rapid detection of acetaminophen (APAP). Blood serum samples were diluted 100-fold with 10 mM ammonium formate/ethanol (1:1 v/v) solution including deuterium-labeled internal standards (IS; APAP-d4). Only 10 μL of the diluted sample was used for measurement. The tandem mass spectrometer (MS/MS) equipped with a PESI was used in selected reaction monitoring mode for the quantitation of APAP; the measurement time was only 18 s. Transitions were set at 152 > 110 for quantitation, 152 > 65 for qualifier, and 156 > 114 for IS (APAP-d4). All measurements were conducted in positive mode. The calibration curve (1/x

Identifiants

pubmed: 31324294
pii: j.jfda.2019.02.001
doi: 10.1016/j.jfda.2019.02.001
pmc: PMC9307038
doi:

Substances chimiques

Analgesics, Non-Narcotic 0
Acetaminophen 362O9ITL9D

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

786-792

Informations de copyright

Copyright © 2019. Published by Elsevier Taiwan LLC.

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Auteurs

Kiyotaka Usui (K)

Division of Forensic Medicine, Tohoku University Graduate School of Medicine, Sendai, 980-8575, Japan.

Haruka Kobayashi (H)

Division of Forensic Medicine, Tohoku University Graduate School of Medicine, Sendai, 980-8575, Japan.

Yuji Fujita (Y)

Division of Emergency Medicine, Iwate Medical University, Morioka, 020-8505, Japan.

Eito Kubota (E)

Division of Forensic Medicine, Tohoku University Graduate School of Medicine, Sendai, 980-8575, Japan.

Tomoki Hanazawa (T)

Emergency Medical Center and Poison Center, Saitama Medical University Hospital, Saitama, 350-0495, Japan.

Tomohiro Yoshizawa (T)

Emergency Medical Center and Poison Center, Saitama Medical University Hospital, Saitama, 350-0495, Japan.

Yoshito Kamijo (Y)

Emergency Medical Center and Poison Center, Saitama Medical University Hospital, Saitama, 350-0495, Japan.

Masato Funayama (M)

Division of Forensic Medicine, Tohoku University Graduate School of Medicine, Sendai, 980-8575, Japan.

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Classifications MeSH