Separation and characterization of unknown impurities in latamoxef sodium by LC-Q-TOF MS and a summary of their positive-ion fragmentation regularities.


Journal

Journal of pharmaceutical and biomedical analysis
ISSN: 1873-264X
Titre abrégé: J Pharm Biomed Anal
Pays: England
ID NLM: 8309336

Informations de publication

Date de publication:
25 Oct 2019
Historique:
received: 08 05 2019
revised: 23 07 2019
accepted: 24 07 2019
pubmed: 5 8 2019
medline: 28 1 2020
entrez: 5 8 2019
Statut: ppublish

Résumé

A simple and sensitive method was developed for separation and characterization of seventeen impurities from commercial latamoxef sodium for injection by liquid chromatography combined with electrospray ionization and QTOF mass spectrometer (LC-ESI-QTOF MS). The chromatographic separation was performed on a Boston Green ODS-AQ C18 column (250 mm × 4.6 mm, 5 μm) under gradient mode using binary mobile phase: (A) ammonium acetate (10 mM)-methanol (99:1, v/v) and (B) ammonium acetate (10 mM)-methanol (70:30, v/v). Based on tandem multistage MS and high resolution MS data, the molecular formulas and structures of unknown impurities were inferred. A plausible formation mechanism of impurities was also proposed. In addition, the fragmentation regularity of degraded impurities in positive-ion mode was summarized.

Identifiants

pubmed: 31377652
pii: S0731-7085(19)31113-6
doi: 10.1016/j.jpba.2019.112793
pii:
doi:

Substances chimiques

Acetates 0
Ions 0
Sodium 9NEZ333N27
ammonium acetate RRE756S6Q2
Moxalactam VUF6C936Z3
Methanol Y4S76JWI15

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

112793

Informations de copyright

Copyright © 2019 Elsevier B.V. All rights reserved.

Auteurs

Lulu He (L)

Zhejiang University of Technology, Hangzhou 310004, China.

Jianqin Qian (J)

Zhejiang Institute for Food and Drug Control, Hangzhou 310052, China.

Peixi Zhu (P)

Zhejiang University of Technology, Hangzhou 310004, China.

Weifeng Yang (W)

Zhejiang Institute for Food and Drug Control, Hangzhou 310052, China. Electronic address: ywfhz@163.com.

Yuanbin She (Y)

Zhejiang University of Technology, Hangzhou 310004, China. Electronic address: sheyb@zjut.edu.cn.

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Classifications MeSH