Inhibition of dual-specificity tyrosine phosphorylation-regulated kinase 2 perturbs 26S proteasome-addicted neoplastic progression.


Journal

Proceedings of the National Academy of Sciences of the United States of America
ISSN: 1091-6490
Titre abrégé: Proc Natl Acad Sci U S A
Pays: United States
ID NLM: 7505876

Informations de publication

Date de publication:
03 12 2019
Historique:
pubmed: 23 11 2019
medline: 2 4 2020
entrez: 23 11 2019
Statut: ppublish

Résumé

Dependence on the 26S proteasome is an Achilles' heel for triple-negative breast cancer (TNBC) and multiple myeloma (MM). The therapeutic proteasome inhibitor, bortezomib, successfully targets MM but often leads to drug-resistant disease relapse and fails in breast cancer. Here we show that a 26S proteasome-regulating kinase, DYRK2, is a therapeutic target for both MM and TNBC. Genome editing or small-molecule mediated inhibition of DYRK2 significantly reduces 26S proteasome activity, bypasses bortezomib resistance, and dramatically delays in vivo tumor growth in MM and TNBC thereby promoting survival. We further characterized the ability of LDN192960, a potent and selective DYRK2-inhibitor, to alleviate tumor burden in vivo. The drug docks into the active site of DYRK2 and partially inhibits all 3 core peptidase activities of the proteasome. Our results suggest that targeting 26S proteasome regulators will pave the way for therapeutic strategies in MM and TNBC.

Identifiants

pubmed: 31754034
pii: 1912033116
doi: 10.1073/pnas.1912033116
pmc: PMC6900511
doi:

Substances chimiques

Proteasome Inhibitors 0
Bortezomib 69G8BD63PP
Protein-Tyrosine Kinases EC 2.7.10.1
TYK2 Kinase EC 2.7.10.2
Protein Serine-Threonine Kinases EC 2.7.11.1
PSMB5 protein, human EC 3.4.25.1
PSMC4 protein, human EC 3.4.25.1
Proteasome Endopeptidase Complex EC 3.4.25.1
ATP dependent 26S protease EC 3.4.99.-
ATPases Associated with Diverse Cellular Activities EC 3.6.4.-

Banques de données

PDB
['6K0J']

Types de publication

Journal Article Research Support, N.I.H., Extramural Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

24881-24891

Subventions

Organisme : NIGMS NIH HHS
ID : R01 GM074024
Pays : United States
Organisme : NLM NIH HHS
ID : T15 LM011271
Pays : United States
Organisme : NCI NIH HHS
ID : U24 CA194107
Pays : United States
Organisme : Cancer Research UK
ID : C52419/A22869
Pays : United Kingdom

Informations de copyright

Copyright © 2019 the Author(s). Published by PNAS.

Déclaration de conflit d'intérêts

The authors declare no competing interest.

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Auteurs

Sourav Banerjee (S)

Department of Pharmacology, University of California San Diego, La Jolla, CA 92093.

Tiantian Wei (T)

The State Key Laboratory of Protein and Plant Gene Research, School of Life Sciences, Peking University, 100871 Beijing, China.
Peking-Tsinghua Center for Life Sciences, Peking University, 100871 Beijing, China.

Jue Wang (J)

Beijing National Laboratory for Molecular Sciences, Key Laboratory of Bioorganic Chemistry and Molecular Engineering of Ministry of Education, College of Chemistry and Molecular Engineering, Peking University, 100871 Beijing, China.

Jenna J Lee (JJ)

Department of Bioengineering, University of California San Diego, La Jolla, CA 92093.

Haydee L Gutierrez (HL)

Division of Biological Sciences, Section of Cellular and Developmental Biology, University of California San Diego, La Jolla, CA 92093.

Owen Chapman (O)

Department of Medicine, University of California San Diego, La Jolla, CA 92093.

Sandra E Wiley (SE)

Department of Pharmacology, University of California San Diego, La Jolla, CA 92093.

Joshua E Mayfield (JE)

Department of Pharmacology, University of California San Diego, La Jolla, CA 92093.

Vasudha Tandon (V)

Department of Pharmacology, University of California San Diego, La Jolla, CA 92093.

Edwin F Juarez (EF)

Department of Medicine, University of California San Diego, La Jolla, CA 92093.

Lukas Chavez (L)

Department of Medicine, University of California San Diego, La Jolla, CA 92093.
Moores Cancer Center, University of California San Diego, La Jolla, CA 92093.

Ruqi Liang (R)

The State Key Laboratory of Protein and Plant Gene Research, School of Life Sciences, Peking University, 100871 Beijing, China.
Peking-Tsinghua Center for Life Sciences, Peking University, 100871 Beijing, China.

Robert L Sah (RL)

Department of Bioengineering, University of California San Diego, La Jolla, CA 92093.

Caitlin Costello (C)

Moores Cancer Center, University of California San Diego, La Jolla, CA 92093.
Division of Blood and Marrow Transplant, University of California San Diego, La Jolla, CA 92093.

Jill P Mesirov (JP)

Department of Medicine, University of California San Diego, La Jolla, CA 92093.
Moores Cancer Center, University of California San Diego, La Jolla, CA 92093.

Laureano de la Vega (L)

Division of Cellular Medicine, School of Medicine, University of Dundee, Dundee, DD1 9SY, United Kingdom.

Kimberly L Cooper (KL)

Division of Biological Sciences, Section of Cellular and Developmental Biology, University of California San Diego, La Jolla, CA 92093.

Jack E Dixon (JE)

Department of Pharmacology, University of California San Diego, La Jolla, CA 92093; jedixon@ucsd.edu junyuxiao@pku.edu.cn xglei@pku.edu.cn.
Department of Cellular and Molecular Medicine, University of California San Diego, La Jolla, CA 92093.
Department of Chemistry and Biochemistry, University of California San Diego, La Jolla, CA 92093.

Junyu Xiao (J)

The State Key Laboratory of Protein and Plant Gene Research, School of Life Sciences, Peking University, 100871 Beijing, China; jedixon@ucsd.edu junyuxiao@pku.edu.cn xglei@pku.edu.cn.
Peking-Tsinghua Center for Life Sciences, Peking University, 100871 Beijing, China.

Xiaoguang Lei (X)

Peking-Tsinghua Center for Life Sciences, Peking University, 100871 Beijing, China; jedixon@ucsd.edu junyuxiao@pku.edu.cn xglei@pku.edu.cn.
Beijing National Laboratory for Molecular Sciences, Key Laboratory of Bioorganic Chemistry and Molecular Engineering of Ministry of Education, College of Chemistry and Molecular Engineering, Peking University, 100871 Beijing, China.
Department of Chemical Biology, Synthetic and Functional Biomolecules Center, Peking University, 100871 Beijing, China.

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Classifications MeSH