Carboxymethyl cellulose/diclofenac bioactive coatings on AISI 316LVM for controlled drug delivery, and improved osteogenic potential.


Journal

Carbohydrate polymers
ISSN: 1879-1344
Titre abrégé: Carbohydr Polym
Pays: England
ID NLM: 8307156

Informations de publication

Date de publication:
15 Feb 2020
Historique:
received: 29 08 2019
revised: 11 10 2019
accepted: 12 11 2019
entrez: 1 1 2020
pubmed: 1 1 2020
medline: 5 6 2020
Statut: ppublish

Résumé

This work reports on the preparation and systematic testing of a novel multi-layered coating, comprised of the non-steroid anti-inflammatory drug diclofenac and biopolymer carboxymethyl cellulose. Drug release testing was performed on an Automated Transdermal Diffusion Cells Sampling System in combination with UV-VIS spectroscopy as the released drug concentration determination method. The results showed that most of the drug is released in the first six hours, whereas the overall released amount could be tailored through changes in the multi-layered coating composition. Biocompatibility tests performed on human osteoblast cells, showed cell viability improvement between 7% and 17% compared to the control sample. The expression of proteins playing important roles in extracellular matrix production and functioning was performed in order to obtain additional proof of the prepared materials' osteointegration boosting capacity. Finally, electrochemical measurements confirmed that the coatings do not influence the corrosion susceptibility of AISI 316LVM stainless steel.

Identifiants

pubmed: 31887952
pii: S0144-8617(19)31280-9
doi: 10.1016/j.carbpol.2019.115612
pii:
doi:

Substances chimiques

Anti-Inflammatory Agents, Non-Steroidal 0
Biocompatible Materials 0
Bone Morphogenetic Protein 2 0
Extracellular Matrix Proteins 0
Proteoglycans 0
osteoadherin 0
Steel 12597-69-2
Diclofenac 144O8QL0L1
Carboxymethylcellulose Sodium K679OBS311

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

115612

Informations de copyright

Copyright © 2019 Elsevier Ltd. All rights reserved.

Auteurs

Uroš Maver (U)

University of Maribor, Faculty of Medicine, Department of Pharmacology, Taborska ulica 8, 2000 Maribor, Slovenia; University of Maribor, Faculty of Medicine, Institute of Biomedical Sciences, Taborska ulica 8, 2000 Maribor, Slovenia. Electronic address: uros.maver@um.si.

Klodian Xhanari (K)

University of Maribor, Faculty of Chemistry and Chemical Engineering, Laboratory for Analytical Chemistry and Industrial Analysis, Smetanova ulica 17,2000 Maribor, Slovenia; University of Tirana, Faculty of Natural Sciences, Boulevard "Zogu I", 1001 Tirana, Albania.

Marko Žižek (M)

University of Maribor, Faculty of Chemistry and Chemical Engineering, Laboratory for Analytical Chemistry and Industrial Analysis, Smetanova ulica 17,2000 Maribor, Slovenia.

Lidija Gradišnik (L)

University of Maribor, Faculty of Medicine, Institute of Biomedical Sciences, Taborska ulica 8, 2000 Maribor, Slovenia.

Katja Repnik (K)

University of Maribor, Faculty of Medicine, Center for Human Molecular Genetics and Pharmacogenomics, Taborska ulica 8, 2000 Maribor, Slovenia; University of Maribor, Faculty for Chemistry and Chemical Engineering, Laboratory for Biochemistry, Molecular Biology and Genomics, Smetanova 17, 2000 Maribor, Slovenia.

Uroš Potočnik (U)

University of Maribor, Faculty of Medicine, Center for Human Molecular Genetics and Pharmacogenomics, Taborska ulica 8, 2000 Maribor, Slovenia; University of Maribor, Faculty for Chemistry and Chemical Engineering, Laboratory for Biochemistry, Molecular Biology and Genomics, Smetanova 17, 2000 Maribor, Slovenia.

Matjaž Finšgar (M)

University of Maribor, Faculty of Chemistry and Chemical Engineering, Laboratory for Analytical Chemistry and Industrial Analysis, Smetanova ulica 17,2000 Maribor, Slovenia. Electronic address: matjaz.finsgar@um.si.

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Classifications MeSH