Direct conversion of wet sewage sludge to carbon catalyst for sulfamethoxazole degradation through peroxymonosulfate activation.

Advanced oxidation process Hydrothermal treatment Ketonic group Water content Wet sludge

Journal

The Science of the total environment
ISSN: 1879-1026
Titre abrégé: Sci Total Environ
Pays: Netherlands
ID NLM: 0330500

Informations de publication

Date de publication:
01 Aug 2020
Historique:
received: 12 02 2020
revised: 15 04 2020
accepted: 18 04 2020
pubmed: 1 5 2020
medline: 11 7 2020
entrez: 1 5 2020
Statut: ppublish

Résumé

The high moisture content of wet sewage sludge generated from wastewater treatment process not only brings high cost of sewage disposal, but also limits its utilization as resource. In this study, an efficient strategy of directly utilizing wet sludge to develop advanced carbocatalyst via a hydrothermal coupled pyrolysis process was proposed. The possible application of as-synthesized carbocatalyst was evaluated by activating peroxymonosulfate (PMS) to degrade a model pollutant of sulfamethoxazole (SMX). Experimental results showed that about 100% of SMX and 59% of total organic carbon (TOC) could be removed within 15 min. Moisture content in wet sludge also affected the performances of as-obtained carbocatalysts. Further studies verified that singlet oxygen (

Identifiants

pubmed: 32353802
pii: S0048-9697(20)32370-6
doi: 10.1016/j.scitotenv.2020.138853
pii:
doi:

Substances chimiques

Peroxides 0
Sewage 0
Water Pollutants, Chemical 0
peroxymonosulfate 22047-43-4
Carbon 7440-44-0
Sulfamethoxazole JE42381TNV

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

138853

Informations de copyright

Copyright © 2020 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Wanrong Hu (W)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China.

Jiangtao Tan (J)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China.

Guohua Pan (G)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China.

Jie Chen (J)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China.

Yundi Chen (Y)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China.

Yi Xie (Y)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China.

Yabo Wang (Y)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China.

Yongkui Zhang (Y)

Department of Pharmaceutical & Biological Engineering, School of Chemical Engineering, Sichuan University, Chengdu 610065, China. Electronic address: zhangyongkui@scu.edu.cn.

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Classifications MeSH