Self-Healing Properties of Bioinspired Amorphous CaCO

3-point bending Portland cement amorphous calcium carbonate calcite microcrack formation nanoindentation polyphosphate self-healing

Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
19 May 2020
Historique:
received: 24 04 2020
revised: 13 05 2020
accepted: 15 05 2020
entrez: 23 5 2020
pubmed: 23 5 2020
medline: 11 2 2021
Statut: epublish

Résumé

There is a strong interest in cement additives that are able to prevent or mitigate the adverse effects of cracks in concrete that cause corrosion of the reinforcement. Inorganic polyphosphate (polyP), a natural polymer that is synthesized by bacteria, even those on cement/concrete, can increase the resistance of concrete to progressive damage from micro-cracking. Here we use a novel bioinspired strategy based on polyP-stabilized amorphous calcium carbonate (ACC) to give this material self-healing properties. Portland cement was supplemented with ACC nanoparticles which were stabilized with 10% (

Identifiants

pubmed: 32438652
pii: molecules25102360
doi: 10.3390/molecules25102360
pmc: PMC7287741
pii:
doi:

Substances chimiques

Glass Ionomer Cements 0
Polyphosphates 0
Calcium Carbonate H0G9379FGK

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : EU Horizon 2020 programme
ID : 760858

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Auteurs

Emad Tolba (E)

ERC Advanced Investigator Grant Research Group at the Institute for Physiological Chemistry, University Medical Center of the Johannes Gutenberg University, Duesbergweg 6, 55128 Mainz, Germany.
Polymers and Pigments Department, National Research Center, Dokki, Giza 12622, Egypt.

Shunfeng Wang (S)

ERC Advanced Investigator Grant Research Group at the Institute for Physiological Chemistry, University Medical Center of the Johannes Gutenberg University, Duesbergweg 6, 55128 Mainz, Germany.

Xiaohong Wang (X)

ERC Advanced Investigator Grant Research Group at the Institute for Physiological Chemistry, University Medical Center of the Johannes Gutenberg University, Duesbergweg 6, 55128 Mainz, Germany.

Meik Neufurth (M)

ERC Advanced Investigator Grant Research Group at the Institute for Physiological Chemistry, University Medical Center of the Johannes Gutenberg University, Duesbergweg 6, 55128 Mainz, Germany.

Maximilian Ackermann (M)

Institute of Functional and Clinical Anatomy, University Medical Center of the Johannes Gutenberg University, Johann Joachim Becher Weg 13, 55099 Mainz, Germany.

Rafael Muñoz-Espí (R)

Institute of Materials Science (ICMUV), Universitat de València, C/Catedràtic José Beltrán 2, 46980 Paterna, València, Spain.

Bothaina M Abd El-Hady (BM)

Polymers and Pigments Department, National Research Center, Dokki, Giza 12622, Egypt.

Heinz C Schröder (HC)

ERC Advanced Investigator Grant Research Group at the Institute for Physiological Chemistry, University Medical Center of the Johannes Gutenberg University, Duesbergweg 6, 55128 Mainz, Germany.
NanotecMARIN GmbH, Mühlstr. 19, 55218 Ingelheim am Rhein, Germany.

Werner E G Müller (WEG)

ERC Advanced Investigator Grant Research Group at the Institute for Physiological Chemistry, University Medical Center of the Johannes Gutenberg University, Duesbergweg 6, 55128 Mainz, Germany.

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Classifications MeSH