Activation of persulfate by graphitized biochar for sulfamethoxazole removal: The roles of graphitic carbon structure and carbonyl group.

Adsorption Advanced oxidation processes Degradation Graphitized biochar Persulfate Sulfamethoxazole

Journal

Journal of colloid and interface science
ISSN: 1095-7103
Titre abrégé: J Colloid Interface Sci
Pays: United States
ID NLM: 0043125

Informations de publication

Date de publication:
01 Oct 2020
Historique:
received: 10 02 2020
revised: 22 05 2020
accepted: 24 05 2020
pubmed: 7 6 2020
medline: 22 6 2021
entrez: 7 6 2020
Statut: ppublish

Résumé

Recently, the application of cheap, easily available biochar (BC) in advanced oxidation processes (AOPs) has received widespread attention. However, it is still a challenge to seek effective modification methods to prepare BC with high catalytic performance. In this study, a novel and environmentally friendly graphitized BC (WGBC) derived from wood chip was prepared, which exhibited excellent performance towards persulfate (PS) activation for sulfamethoxazole (SMX) removal as compared to original BC. Series characterizations confirmed that such improved catalytic performance was attributed to the well-established graphitic carbon structure and surface functionalized CO group. Free radical quenching and electron paramagnetic resonance (EPR) experiments qualitatively demonstrated that SO

Identifiants

pubmed: 32505002
pii: S0021-9797(20)30706-2
doi: 10.1016/j.jcis.2020.05.096
pii:
doi:

Substances chimiques

Water Pollutants, Chemical 0
biochar 0
Charcoal 16291-96-6
Carbon 7440-44-0
Graphite 7782-42-5
Sulfamethoxazole JE42381TNV

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

419-430

Informations de copyright

Copyright © 2020 Elsevier Inc. All rights reserved.

Auteurs

Li Du (L)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China; Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, China.

Weihua Xu (W)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China; Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, China. Electronic address: whxu@hnu.edu.cn.

Shaobo Liu (S)

School of Metallurgy and Environment, Central South University, Lushan South Road, Yuelu District, Changsha 410083, China. Electronic address: liushaobo@csu.edu.cn.

Xin Li (X)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China; Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, China.

Danlian Huang (D)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China; Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, China.

Xiaofei Tan (X)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China; Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, China.

Yunguo Liu (Y)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China; Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, China.

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Classifications MeSH