Effects of EDTA on adsorption of Cd(II) and Pb(II) by soil minerals in low-permeability layers: batch experiments and microscopic characterization.
Adsorption capacity
Clay
EDTA
Heavy metals
Low-molecular-weight organic acids
Low-permeability
Journal
Environmental science and pollution research international
ISSN: 1614-7499
Titre abrégé: Environ Sci Pollut Res Int
Pays: Germany
ID NLM: 9441769
Informations de publication
Date de publication:
Nov 2020
Nov 2020
Historique:
received:
23
04
2020
accepted:
15
07
2020
pubmed:
22
7
2020
medline:
3
11
2020
entrez:
22
7
2020
Statut:
ppublish
Résumé
Ethylenediaminetetraacetic acid (EDTA) can serve as a washing agent in the remediation of low-permeability layers contaminated by heavy metals (HMs). Therefore, batch adsorption experiments, where pure quartz (SM1) and mineral mixtures (SM2) were used as typical soil minerals (SMs) in low-permeability layers, were implemented to explore the effects of different EDTA concentrations, pH, and exogenous chemicals on the HM-SM-EDTA adsorption system. As the EDTA concentration increased, it gradually cut down the maximum Cd adsorption capacities of SM1 and SM2 from approximately 135 to 55 mg/kg and 2660 to 1453 mg/kg; and the maximum Pb adsorption capacities of SM1 and SM2 were reduced from 660 to 306 mg/kg and 19,677 to 19,262 mg/kg, respectively. When the initial mole ratio (MR = moles of HM ions/sum of moles of HM ions and EDTA) was closer to 0.5, the effect of EDTA was more effective. Additionally, EDTA worked well at pH below 7.0 and 4.0 for Cd and Pb, respectively. Low-molecular-weight organic acids (LMWOAs) affected the system mainly by bridging, complexation, adsorption site competition, and reductive dissolution. Cu
Identifiants
pubmed: 32691313
doi: 10.1007/s11356-020-10149-9
pii: 10.1007/s11356-020-10149-9
doi:
Substances chimiques
Metals, Heavy
0
Minerals
0
Soil
0
Soil Pollutants
0
Cadmium
00BH33GNGH
Lead
2P299V784P
Edetic Acid
9G34HU7RV0
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
41623-41638Subventions
Organisme : National Natural Science Foundation of China
ID : 41672230, 51961145106
Organisme : National Natural Science Foundation of China
ID : 41601514
Organisme : Shanghai science and technology innovation action plan project
ID : 19ZR1459300,19230742400
Organisme : the Interdisciplinarity Fund of Peak Discipline from Shanghai Municipal Education Commission
ID : 0200121005/053, 2019010202
Organisme : Key Laboratory of Yangtze River Water Environment for Ministry of Education, Tongji University
ID : YRWEF201604
Organisme : State Key Laboratory of Petroleum Pollution Control
ID : PPC2016019
Organisme : the International Exchange Program for Graduate Students, Tongji University
ID : 201902053
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