HONO Budget and Its Role in Nitrate Formation in the Rural North China Plain.


Journal

Environmental science & technology
ISSN: 1520-5851
Titre abrégé: Environ Sci Technol
Pays: United States
ID NLM: 0213155

Informations de publication

Date de publication:
15 09 2020
Historique:
pubmed: 19 8 2020
medline: 15 12 2020
entrez: 19 8 2020
Statut: ppublish

Résumé

Nitrous acid (HONO) is a major precursor of tropospheric hydroxyl radical (OH) that accelerates the formation of secondary pollutants. The HONO sources, however, are not well understood, especially in polluted areas. Based on a comprehensive winter field campaign conducted at a rural site of the North China Plain, a box model (MCM v3.3.1) was used to simulate the daytime HONO budget and nitrate formation. We found that HONO photolysis acted as the dominant source for primary OH with a contribution of more than 92%. The observed daytime HONO could be well explained by the known sources in the model. The heterogeneous conversion of NO

Identifiants

pubmed: 32808764
doi: 10.1021/acs.est.0c01832
doi:

Substances chimiques

Aerosols 0
Nitrates 0
Hydroxyl Radical 3352-57-6
Nitrous Acid T2I5UM75DN

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

11048-11057

Auteurs

Chaoyang Xue (C)

Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace (LPC2E), CNRS-Université Orléans-CNES, 45071 Orléans Cedex 2, France.
University of Chinese Academy of Sciences, Beijing 100049, China.

Chenglong Zhang (C)

Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
Centre for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

Can Ye (C)

Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

Pengfei Liu (P)

Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
Centre for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

Valéry Catoire (V)

Laboratoire de Physique et Chimie de l'Environnement et de l'Espace (LPC2E), CNRS-Université Orléans-CNES, 45071 Orléans Cedex 2, France.

Gisèle Krysztofiak (G)

Laboratoire de Physique et Chimie de l'Environnement et de l'Espace (LPC2E), CNRS-Université Orléans-CNES, 45071 Orléans Cedex 2, France.

Hui Chen (H)

Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai 200438, China.

Yangang Ren (Y)

Institut de Combustion Aérothermique, Réactivité et Environnement, Centre National de la Recherche Scientifique (ICARE-CNRS), Observatoire des Sciences de l'Univers en région Centre, CS 50060, 45071 Orléans Cedex 2, France.

Xiaoxi Zhao (X)

Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

Jinhe Wang (J)

School of Municipal and Environmental Engineering, Co-Innovation Centre for Green Building of Shandong Province, Shandong Jianzhu University, Jinan 250101, China.

Fei Zhang (F)

Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai 200438, China.

Chongxu Zhang (C)

School of Municipal and Environmental Engineering, Co-Innovation Centre for Green Building of Shandong Province, Shandong Jianzhu University, Jinan 250101, China.

Jingwei Zhang (J)

University of Chinese Academy of Sciences, Beijing 100049, China.
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics (IAP), Chinese Academy of Sciences, Beijing 100029, China.

Junling An (J)

University of Chinese Academy of Sciences, Beijing 100049, China.
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics (IAP), Chinese Academy of Sciences, Beijing 100029, China.

Tao Wang (T)

Department of Civil and Environmental Engineering, Hong Kong Polytechnic University, Hong Kong, China.

Jianmin Chen (J)

Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai 200438, China.

Jörg Kleffmann (J)

Physical and Theoretical Chemistry, University of Wuppertal, Gaußstrasse 20, 42119 Wuppertal, Germany.

Abdelwahid Mellouki (A)

Institut de Combustion Aérothermique, Réactivité et Environnement, Centre National de la Recherche Scientifique (ICARE-CNRS), Observatoire des Sciences de l'Univers en région Centre, CS 50060, 45071 Orléans Cedex 2, France.
Environmental Research Institute, Shandong University, Jinan 250100, Shandong, China.

Yujing Mu (Y)

Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
Centre for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China.
University of Chinese Academy of Sciences, Beijing 100049, China.

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