Discovery of potent small molecule PROTACs targeting mutant EGFR.


Journal

European journal of medicinal chemistry
ISSN: 1768-3254
Titre abrégé: Eur J Med Chem
Pays: France
ID NLM: 0420510

Informations de publication

Date de publication:
15 Dec 2020
Historique:
received: 25 07 2020
revised: 20 08 2020
accepted: 21 08 2020
pubmed: 5 9 2020
medline: 27 5 2021
entrez: 5 9 2020
Statut: ppublish

Résumé

Epidermal growth factor receptor (EGFR) is an important therapeutic target for the treatment of non-small cell lung cancer. A number of efficacious EGFR tyrosine kinase inhibitors have been developed. However, acquired drug resistance largely encumbered their clinical practicability. Therefore, there is an urgent need to develop new therapeutic regime. Herein, we designed and synthesized a set of EGFR-targeting small molecule PROTACs which showed promising efficacy. In particular, VHL-recruiting compound P3 showed potent anti-proliferative activity against HCC827 and H1975 cell lines with IC

Identifiants

pubmed: 32883633
pii: S0223-5234(20)30753-4
doi: 10.1016/j.ejmech.2020.112781
pii:
doi:

Substances chimiques

Adaptor Proteins, Signal Transducing 0
Antineoplastic Agents 0
CRBN protein, human 0
Protein Kinase Inhibitors 0
Purines 0
Ubiquitin-Protein Ligases EC 2.3.2.27
Von Hippel-Lindau Tumor Suppressor Protein EC 2.3.2.27
EGFR protein, human EC 2.7.10.1
ErbB Receptors EC 2.7.10.1
VHL protein, human EC 6.3.2.-
Lenalidomide F0P408N6V4

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

112781

Informations de copyright

Copyright © 2020 Elsevier Masson SAS. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Hong-Yi Zhao (HY)

Department of Medicinal Chemistry, School of Pharmacy, Xi'an Jiaotong University, Xi'an, Shaanxi, 710061, PR China.

Xue-Yan Yang (XY)

Department of Medicinal Chemistry, School of Pharmacy, Xi'an Jiaotong University, Xi'an, Shaanxi, 710061, PR China.

Hao Lei (H)

Department of Medicinal Chemistry, School of Pharmacy, Xi'an Jiaotong University, Xi'an, Shaanxi, 710061, PR China.

Xiao-Xiao Xi (XX)

Department of Medicinal Chemistry, School of Pharmacy, Xi'an Jiaotong University, Xi'an, Shaanxi, 710061, PR China.

She-Min Lu (SM)

School of Basic Medical Sciences, Xi'an Jiaotong University Health Science Center, Xi'an, Shaanxi, 710061, PR China.

Jun-Jie Zhang (JJ)

School of Science, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, PR China.

Minhang Xin (M)

Department of Medicinal Chemistry, School of Pharmacy, Xi'an Jiaotong University, Xi'an, Shaanxi, 710061, PR China. Electronic address: xmhcpu@163.com.

San-Qi Zhang (SQ)

Department of Medicinal Chemistry, School of Pharmacy, Xi'an Jiaotong University, Xi'an, Shaanxi, 710061, PR China. Electronic address: sqzhang@xjtu.edu.cn.

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Classifications MeSH