Synthesis and Evaluation of Voltage-Gated Sodium Channel Blocking Pyrroline Derivatives Endowed with Both Antiarrhythmic and Antioxidant Activities.


Journal

ChemMedChem
ISSN: 1860-7187
Titre abrégé: ChemMedChem
Pays: Germany
ID NLM: 101259013

Informations de publication

Date de publication:
04 02 2021
Historique:
received: 04 09 2020
pubmed: 6 10 2020
medline: 11 11 2021
entrez: 5 10 2020
Statut: ppublish

Résumé

Under the hypothesis that cardioprotective agents might benefit from synergism between antiarrhythmic activity and antioxidant properties, a small series of mexiletine analogues were coupled with the 2,2,5,5-tetramethylpyrroline moiety, known for its antioxidant effect, in order to obtain dual-acting drugs potentially useful in the protection of the heart against post-ischemic reperfusion injury. The pyrroline derivatives reported herein were found to be more potent as antiarrhythmic agents than mexiletine and displayed antioxidant activity. The most interesting tetramethylpyrroline congener, a tert-butyl-substituted analogue, was at least 100 times more active as an antiarrhythmic than mexiletine.

Identifiants

pubmed: 33015979
doi: 10.1002/cmdc.202000692
doi:

Substances chimiques

Anti-Arrhythmia Agents 0
Antioxidants 0
Fluoresceins 0
Pyrroles 0
Voltage-Gated Sodium Channel Blockers 0
Voltage-Gated Sodium Channels 0
2',7'-dichlorodihydrofluorescein 106070-31-9
pyrroline 28350-87-0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

578-588

Subventions

Organisme : University of Bari Aldo Moro

Informations de copyright

© 2020 Wiley-VCH GmbH.

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Auteurs

Alessia Carocci (A)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Mariagrazia Roselli (M)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Roberta Budriesi (R)

Department of Pharmacy and Biotechnologies, Alma Mater Studiorum-University of Bologna, Via Belmeloro 6, Bologna, 40126, Italy.

Matteo Micucci (M)

Department of Pharmacy and Biotechnologies, Alma Mater Studiorum-University of Bologna, Via Belmeloro 6, Bologna, 40126, Italy.

Jean-François Desaphy (JF)

Department of Biomedical Sciences and Human Oncology, University of Bari Aldo Moro, piazza Giulio Cesare, 70126, Bari, Italy.

Concetta Altamura (C)

Department of Biomedical Sciences and Human Oncology, University of Bari Aldo Moro, piazza Giulio Cesare, 70126, Bari, Italy.

Maria Maddalena Cavalluzzi (MM)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Maddalena Toma (M)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Giovanna Ilaria Passeri (GI)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Gualtiero Milani (G)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Angelo Lovece (A)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Alessia Catalano (A)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Claudio Bruno (C)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Annalisa De Palma (A)

Department of Biosciences, Biotechnologies and Biopharmaceutics, University of Bari Aldo Moro, via E. Orabona 4, 70126, Bari, Italy.

Filomena Corbo (F)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Carlo Franchini (C)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

Solomon Habtemariam (S)

Pharmacognosy Research Laboratories & Herbal Analysis services UK, University of Greenwich, Chatham-Maritime, Kent, ME4 4TB, UK.

Giovanni Lentini (G)

Department of Pharmacy - Pharmaceutical Sciences, University of Bari Aldo Moro, via E. Orabona n. 4, 70126, Bari, Italy.

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