Persulfate assisted hydrothermal processing of spirulina for enhanced deoxidation carbonization.

Carbon Carbonization Hydrochar Hydrothermal processing Persulfate Spirulina

Journal

Bioresource technology
ISSN: 1873-2976
Titre abrégé: Bioresour Technol
Pays: England
ID NLM: 9889523

Informations de publication

Date de publication:
Feb 2021
Historique:
received: 05 11 2020
revised: 08 12 2020
accepted: 09 12 2020
pubmed: 22 12 2020
medline: 8 1 2021
entrez: 21 12 2020
Statut: ppublish

Résumé

The influence of persulfate assisted hydrothermal carbonization (HTC) (160 °C-220 °C) of spirulina and hydrochar properties was assessed. The elementary composition and proximate analysis of hydrochar were investigated on the carbonization degree and basic fuel properties, and the surface functional groups and morphological characteristics of hydrochar were analyzed as well as thermal stability. Results suggested that persulfate assisted process enhanced the carbonization degree of hydrochar by oxygen reduction (1.53%-2.74%) and increase of C ratio, and HHVs increased 0.81-1.39 MJ/kg at temperature above 180 °C. The -OH and CO on hydrochar surface were significantly reduced, and C-(C, H) and C-(O, N) were weakened by persulfate addition and more C-H peaks was formed. Additionally, the persulfate addition enhanced the thermal stability of hydrochar by lowing the maximum mass loss rate. The result suggested that HTC can be conducted with persulfate at lower temperature for hydrochar biofuel production.

Identifiants

pubmed: 33348116
pii: S0960-8524(20)31817-4
doi: 10.1016/j.biortech.2020.124543
pii:
doi:

Substances chimiques

Biofuels 0
Carbon 7440-44-0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

124543

Informations de copyright

Copyright © 2020 Elsevier Ltd. All rights reserved.

Auteurs

Tengfei Wang (T)

Faculty of Geosciences and Environmental Engineering, Southwest Jiaotong University, Chengdu 611756, China. Electronic address: wtfgxp@163.com.

Xiangmin Liu (X)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China.

Dongmei Wang (D)

Faculty of Geosciences and Environmental Engineering, Southwest Jiaotong University, Chengdu 611756, China.

Zhengjun Gong (Z)

Faculty of Geosciences and Environmental Engineering, Southwest Jiaotong University, Chengdu 611756, China. Electronic address: gongzhengjun@126.com.

Buchun Si (B)

Laboratory of Environment-Enhancing Energy (E2E), Key Laboratory of Agricultural Engineering in Structure and Environment, Ministry of Agriculture, College of Water Resources and Civil Engineering, China Agricultural University, Beijing 100083, China.

Yunbo Zhai (Y)

College of Environmental Science and Engineering, Hunan University, Changsha 410082, China.

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