The degradation of acetaldehyde in estuary waters in Southern California, USA.
Acetaldehyde,
Bacteria,
Degradation,
Estuary,
Southern California
Turnover,
Journal
Environmental science and pollution research international
ISSN: 1614-7499
Titre abrégé: Environ Sci Pollut Res Int
Pays: Germany
ID NLM: 9441769
Informations de publication
Date de publication:
Jul 2021
Jul 2021
Historique:
received:
29
12
2020
accepted:
26
02
2021
pubmed:
7
3
2021
medline:
16
7
2021
entrez:
6
3
2021
Statut:
ppublish
Résumé
Acetaldehyde plays an important role in oxidative cycles in the troposphere. Estimates of its air-water flux are important in global models. Biological degradation is believed to be the dominant loss process in water, but there have been few measurements, none in estuaries. Acetaldehyde degradation rates were measured in surface waters at the inflow to the Upper Newport Back Bay estuary in Orange County, Southern California, USA, over a 6-month period including the rainy winter season. Deuterated acetaldehyde was added to filtered and unfiltered water samples incubated in glass syringes, and its loss analyzed by purge and trap gas chromatography mass spectrometry. Filtered samples showed no significant degradation, suggesting that particle-mediated degradation is the dominant removal process. Correlation between measured degradation rate constants in unfiltered incubations and bacteria counts suggests the loss is due to microorganisms. Degradation in unfiltered samples followed first-order kinetics, with rate constants ranging from 0.0006 to 0.025 min
Identifiants
pubmed: 33675494
doi: 10.1007/s11356-021-13232-x
pii: 10.1007/s11356-021-13232-x
doi:
Substances chimiques
Water Pollutants, Chemical
0
Acetaldehyde
GO1N1ZPR3B
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
35811-35821Subventions
Organisme : National Science Foundation
ID : OCE # 1233091
Organisme : National Science Foundation
ID : CHE #1337396
Informations de copyright
© 2021. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.
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