Nitroxide spin labels and EPR spectroscopy: A powerful association for protein dynamics studies.


Journal

Biochimica et biophysica acta. Proteins and proteomics
ISSN: 1878-1454
Titre abrégé: Biochim Biophys Acta Proteins Proteom
Pays: Netherlands
ID NLM: 101731734

Informations de publication

Date de publication:
07 2021
Historique:
received: 31 10 2020
revised: 17 03 2021
accepted: 18 03 2021
pubmed: 25 3 2021
medline: 21 9 2021
entrez: 24 3 2021
Statut: ppublish

Résumé

Site-Directed Spin Labelling (SDSL) technique is based on the attachment of a paramagnetic label onto a specific position of a protein (or other bio-molecules) and the subsequent study by Electron Paramagnetic Resonance (EPR) spectroscopy. In particular, continuous-wave EPR (cw-EPR) spectra can detect the local conformational dynamics for proteins under various conditions. Moreover, pulse-EPR experiments on doubly spin-labelled proteins allow measuring distances between spin centres in the 1.5-8 nm range, providing information about structures and functions. This review focuses on SDSL-EPR spectroscopy as a structural biology tool to investigate proteins using nitroxide labels. The versatility of this spectroscopic approach for protein structural characterization has been demonstrated through the choice of recent studies. The main aim is to provide a general overview of the technique, particularly for non-experts, to spread the applicability of this technique in various fields of structural biology.

Identifiants

pubmed: 33757896
pii: S1570-9639(21)00059-5
doi: 10.1016/j.bbapap.2021.140653
pii:
doi:

Substances chimiques

Nitrogen Oxides 0
Proteins 0
Spin Labels 0
nitroxyl GFQ4MMS07W

Types de publication

Journal Article Research Support, Non-U.S. Gov't Review

Langues

eng

Sous-ensembles de citation

IM

Pagination

140653

Informations de copyright

Copyright © 2021 Elsevier B.V. All rights reserved.

Auteurs

F Torricella (F)

CERM-Magnetic Resonance Center, Department of Chemistry, University of Florence, via L.Sacconi 6, 50019 Sesto Fiorentino, Italy.

A Pierro (A)

Aix Marseille Univ, CNRS, BIP, Bioénergétique et Ingénierie des Protéines, IMM, Marseille, France.

E Mileo (E)

Aix Marseille Univ, CNRS, BIP, Bioénergétique et Ingénierie des Protéines, IMM, Marseille, France.

V Belle (V)

Aix Marseille Univ, CNRS, BIP, Bioénergétique et Ingénierie des Protéines, IMM, Marseille, France.

A Bonucci (A)

CERM-Magnetic Resonance Center, Department of Chemistry, University of Florence, via L.Sacconi 6, 50019 Sesto Fiorentino, Italy; Aix Marseille Univ, CNRS, BIP, Bioénergétique et Ingénierie des Protéines, IMM, Marseille, France. Electronic address: bonucci@cerm.unifi.it.

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Classifications MeSH