Perfluoroalkyl substances (PFASs) in the Ugandan waters of Lake Victoria: Spatial distribution, catchment release and public exposure risk via municipal water consumption.

Perfluoroalkyl substances (PFASs) have scarcely been studied in the Lake Victoria Basin and Africa in general. We investigated spatial profiles of PFASs in the Ugandan part of Lake Victoria, their influxes and human exposure via drinking water. We analyzed open lake water, riverine water (Rivers Kagera and Sio), urban drainage water (Nakivubo Channel), over-lake bulk atmospheric deposition and municipal tap water (Kampala, Jinja and Entebbe). The average concentrations (ng/L) for individual target PFASs were in the ranges of 0.08-23.8 (Nakivubo Channel), 0.01-10.8 (Murchison Bay), <MDL-5.38 (Kampala tap water), 0.01-3.64 (R. Kagera), <MDL-3.56 (Jinja tap water), <MDL-3.35 (R. Sio), <MDL-1.96 (Entebbe tap water), <MDL-1.46 (open lake) and <MDL-1.00 (atmospheric deposition). Estimated contribution of input pathways to ∑PFAS fluxes into Lake Victoria was in the order atmospheric deposition > R. Kagera, >R. Sio > Nakivubo Channel. Perfluorohexanoic acid (PFHxA) and perfluorooctane sulfonic acid (PFOS) had the highest influx and retention estimates, respectively. Perfluoroalkane sulfonates (PFSAs) were mostly associated with urban drainage samples. PFASs were likely recycled from the Nakivubo Channel, through the Murchison Bay, into municipal drinking water. The estimated human exposure to ∑

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Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.