Correlation of Thermoelectric Performance, Domain Morphology and Doping Level in PEDOT:PSS Thin Films Post-Treated with Ionic Liquids.
GISAXS
PEDOT:PSS
ionic liquids
morphology
thermoelectric thin films
Journal
Macromolecular rapid communications
ISSN: 1521-3927
Titre abrégé: Macromol Rapid Commun
Pays: Germany
ID NLM: 9888239
Informations de publication
Date de publication:
Oct 2021
Oct 2021
Historique:
revised:
30
08
2021
received:
24
06
2021
pubmed:
8
9
2021
medline:
27
10
2021
entrez:
7
9
2021
Statut:
ppublish
Résumé
Ionic liquid (IL) post-treatment of poly(3,4-ethylene dioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) thin films with ethyl-3-methylimidazolium dicyanamide (EMIM DCA), allyl-3-methylimidazolium dicyanamide (AMIM DCA), and 1-ethyl-3-methylimidazolium tetracyanoborate (EMIM TCB) is compared. Doping level modifications of PEDOT are characterized using UV-Vis spectroscopy and directly correlate with the observed Seebeck coefficient enhancement. With conductive atomic force microscopy (c-AFM) the authors investigate changes in the topographic-current features of the PEDOT:PSS thin film surface due to IL treatment. Grazing incidence small-angle X-ray scattering (GISAXS) demonstrates the morphological rearrangement towards an optimized PEDOT domain distribution upon IL post-treatment, directly facilitating the interconductivity and causing an increased film conductivity. Based on these improvements in Seebeck coefficient and conductivity, the power factor is increased up to 236 µW m
Identifiants
pubmed: 34491602
doi: 10.1002/marc.202100397
doi:
Substances chimiques
Bridged Bicyclo Compounds, Heterocyclic
0
Ionic Liquids
0
Polymers
0
Polystyrenes
0
poly(3,4-ethylene dioxythiophene)
0
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2100397Subventions
Organisme : Deutsche Forschungsgemeinschaft
ID : EXC 2089/1 - 390776260
Organisme : Bayerische Staatsministerium für Wissenschaft und Kunst: Bavarian Collaborative Research Project Solar Technologies Go Hybrid (SolTech)
Organisme : Center for NanoScience
Organisme : Deutsche Forschungsgemeinschaf: International Research Training Group 2022 Alberta/Technical University of Munich International Graduate School for Environmentally Responsible Functional Hybrid Materials (ATUMS)
Organisme : China Scholarship Council
Informations de copyright
© 2021 The Authors. Macromolecular Rapid Communications published by Wiley-VCH GmbH.
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