Bidirectional Phase Transformation of Supramolecular Networks Using Two Molecular Signals.

bilayer heterostructure molecular self-assembly molecular signaling reversible phase control scanning tunneling microscopy

Journal

ACS nano
ISSN: 1936-086X
Titre abrégé: ACS Nano
Pays: United States
ID NLM: 101313589

Informations de publication

Date de publication:
25 Jan 2022
Historique:
pubmed: 12 1 2022
medline: 11 11 2022
entrez: 11 1 2022
Statut: ppublish

Résumé

Reversible control of molecular self-assembly is omnipresent in adaptive biological systems, yet its realization in artificial systems remains a major challenge. Using scanning tunneling microscopy and density functional theory calculations, we show that a 2D supramolecular network formed by terthienobenzenetricarboxylic acid (TTBTA) can undergo a reversible structural transition between a porous and dense phase in response to different molecular signals (trimethyltripyrazolotriazine (TMTPT) and C

Identifiants

pubmed: 35014801
doi: 10.1021/acsnano.1c10122
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1560-1566

Auteurs

Daling Cui (D)

Department of Chemistry, McGill University 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada.
Centre Énergie, Matériaux et Télécommunications, Institut National de la Recherche Scientifique, 1650 Boulevard Lionel-Boulet, Varennes, Québec J3X 1S2, Canada.

Cheng-Hao Liu (CH)

Department of Chemistry, McGill University 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada.

Federico Rosei (F)

Centre Énergie, Matériaux et Télécommunications, Institut National de la Recherche Scientifique, 1650 Boulevard Lionel-Boulet, Varennes, Québec J3X 1S2, Canada.

Dmitrii F Perepichka (DF)

Department of Chemistry, McGill University 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada.

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Classifications MeSH