Methyltransferases: Functions and Applications.

S-adenosyl-l-methionine biocatalysis enzymes methyltransferases

Journal

Chembiochem : a European journal of chemical biology
ISSN: 1439-7633
Titre abrégé: Chembiochem
Pays: Germany
ID NLM: 100937360

Informations de publication

Date de publication:
16 09 2022
Historique:
revised: 10 06 2022
received: 14 04 2022
pubmed: 13 6 2022
medline: 20 9 2022
entrez: 12 6 2022
Statut: ppublish

Résumé

In this review the current state-of-the-art of S-adenosylmethionine (SAM)-dependent methyltransferases and SAM are evaluated. Their structural classification and diversity is introduced and key mechanistic aspects presented which are then detailed further. Then, catalytic SAM as a target for drugs, and approaches to utilise SAM as a cofactor in synthesis are introduced with different supply and regeneration approaches evaluated. The use of SAM analogues are also described. Finally O-, N-, C- and S-MTs, their synthetic applications and potential for compound diversification is given.

Identifiants

pubmed: 35691829
doi: 10.1002/cbic.202200212
pmc: PMC9539859
doi:

Substances chimiques

S-Adenosylmethionine 7LP2MPO46S
Methyltransferases EC 2.1.1.-

Types de publication

Journal Article Review Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202200212

Subventions

Organisme : Wellcome Trust
ID : 219857/Z/19/Z
Pays : United Kingdom

Informations de copyright

© 2022 The Authors. ChemBioChem published by Wiley-VCH GmbH.

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Auteurs

Eman Abdelraheem (E)

Biocatalysis, Department of Biotechnology, Delft University of Technology, Van der Maasweg 9, 2629 HZ, Delft (The, Netherlands.

Benjamin Thair (B)

Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK.

Romina Fernández Varela (RF)

Laboratorio de Biotransformaciones y Química de Ácidos Nucleicos, Universidad Nacional de Quilmes, Roque S. Peña 352, B1876BXD, Bernal, Argentina.

Emely Jockmann (E)

Institute of Pharmaceutical Sciences, University of Freiburg, Albertstr. 25, 79104, Freiburg, Germany.

Désirée Popadić (D)

Institute of Pharmaceutical Sciences, University of Freiburg, Albertstr. 25, 79104, Freiburg, Germany.

Helen C Hailes (HC)

Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK.

John M Ward (JM)

Department of Biochemical Engineering, Bernard Katz Building, University College London, London, WC1E 6BT, UK.

Adolfo M Iribarren (AM)

Laboratorio de Biotransformaciones y Química de Ácidos Nucleicos, Universidad Nacional de Quilmes, Roque S. Peña 352, B1876BXD, Bernal, Argentina.

Elizabeth S Lewkowicz (ES)

Laboratorio de Biotransformaciones y Química de Ácidos Nucleicos, Universidad Nacional de Quilmes, Roque S. Peña 352, B1876BXD, Bernal, Argentina.

Jennifer N Andexer (JN)

Institute of Pharmaceutical Sciences, University of Freiburg, Albertstr. 25, 79104, Freiburg, Germany.

Peter-Leon Hagedoorn (PL)

Biocatalysis, Department of Biotechnology, Delft University of Technology, Van der Maasweg 9, 2629 HZ, Delft (The, Netherlands.

Ulf Hanefeld (U)

Biocatalysis, Department of Biotechnology, Delft University of Technology, Van der Maasweg 9, 2629 HZ, Delft (The, Netherlands.

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