A feasible approach to tune the interaction of chitosan with sodium dodecyl sulfate.

Chitosan Chitosanpoly[(1 → 4-β)-d-2-amino-2-deoxyglucopyranose] Sodium dodecyl sulfate Cryo-TEM Interaction Nonionic surfactant Sodium dodecyl sulfate Triton X-1002-[4-(2,4,4-trimethylpentan-2-yl)phenoxy]ethanol Triton-30511-(4-tert-octylphenoxy)-3,6,9-trioxaundecane-1-ol Turbodimetry, light scattering Tween 20, Polyoxyethylene (20) sorbitan monolaurate2-[2-[3,4-bis(2-hydroxyethoxy)oxolan-2-yl]-2-(2-hydroxyethoxy)ethoxy]ethyl dodecanoate Tween 80, Polyoxyethylene sorbitan monooleate2-[2-[3,4-bis(2-hydroxyethoxy)oxolan-2-yl]-2-(2-hydroxyethoxy)ethoxy]ethyl (E)-octadec-9-enoate

Journal

Carbohydrate polymers
ISSN: 1879-1344
Titre abrégé: Carbohydr Polym
Pays: England
ID NLM: 8307156

Informations de publication

Date de publication:
15 Sep 2022
Historique:
received: 18 01 2022
revised: 16 05 2022
accepted: 17 05 2022
entrez: 20 6 2022
pubmed: 21 6 2022
medline: 23 6 2022
Statut: ppublish

Résumé

Interaction of binary chitosan/nonionic surfactant (NIS) system with sodium dodecyl sulfate (SDS) in aqueous solution is described using turbodimetry, light scattering, electophoretic mobility and cryogenic electron microscopy. The formation of insoluble CHI/SDS complexes is weakened with a decrease in molecular weight of chitosan and critical micelle concentration of NIS as well as with an increase in NIS concentration. Soluble chitosan/NIS complexes absorb SDS molecules until the charge of mixed chitosan/NIS/SDS complexes reaches a critical value that depends on chitosan molecular weight followed by aggregation of primary electrostatic complexes via hydrogen bonding to complex nanoparticles. In contrast to formation of asymmetric swarm-like structures in the binary chitosan/SDS system, the aggregation of complex nanoparticles in the ternary chitosan/NIS/SDS system occurs by a head-to-tail binding mechanism with formation of elongated filamentous microstructures. The finding can be promising for preparation of microbiologically stable pharmaceutical and cosmetic compositions and drug delivery systems containing mixed surfactants.

Identifiants

pubmed: 35725155
pii: S0144-8617(22)00547-1
doi: 10.1016/j.carbpol.2022.119642
pii:
doi:

Substances chimiques

Micelles 0
Surface-Active Agents 0
Sodium Dodecyl Sulfate 368GB5141J
Chitosan 9012-76-4

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

119642

Informations de copyright

Copyright © 2022 Elsevier Ltd. All rights reserved.

Auteurs

Evgeniya A Bezrodnykh (EA)

A. N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Moscow, Russia.

Boris B Berezin (BB)

A. N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Moscow, Russia.

Yury A Antonov (YA)

N.M. Emanuel Institute of Biochemical Physics, Russian Academy of Sciences, Moscow, Russia.

Irina L Zhuravleva (IL)

N.M. Emanuel Institute of Biochemical Physics, Russian Academy of Sciences, Moscow, Russia.

Anastasia A Atamas (AA)

Moscow Institute of Physics and Technology, Moscow Region, Dolgoprudny, Moscow, Russia.

Aleksei A Tsarenko (AA)

Moscow Institute of Physics and Technology, Moscow Region, Dolgoprudny, Moscow, Russia.

Andrey V Rogachev (AV)

Moscow Institute of Physics and Technology, Moscow Region, Dolgoprudny, Moscow, Russia.

Vladimir E Tikhonov (VE)

A. N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Moscow, Russia. Electronic address: tikhon@ineos.ac.ru.

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Classifications MeSH