Simulating indoor inorganic aerosols of outdoor origin with the inorganic aerosol thermodynamic equilibrium model ISORROPIA.


Journal

Indoor air
ISSN: 1600-0668
Titre abrégé: Indoor Air
Pays: England
ID NLM: 9423515

Informations de publication

Date de publication:
07 2022
Historique:
revised: 31 05 2022
received: 08 12 2021
accepted: 24 06 2022
entrez: 29 7 2022
pubmed: 30 7 2022
medline: 3 8 2022
Statut: ppublish

Résumé

Outdoor aerosols can transform and have their composition altered upon transport indoors. Herein, IMAGES, a platform that simulates indoor organic aerosol with the 2-dimensional volatility basis set (2D-VBS), was extended to incorporate the inorganic aerosol thermodynamic equilibrium model, ISORROPIA. The model performance was evaluated by comparing aerosol component predictions to indoor measurements from an aerosol mass spectrometer taken during the summer and winter seasons. Since ammonia was not measured in the validation dataset, outdoor ammonia was estimated from aerosol measurements using a novel pH-based algorithm, while nitric acid was held constant. Modeled indoor ammonia sources included temperature-based occupant and surface emissions. Sensitivity to the nitric acid indoor surface deposition rate

Identifiants

pubmed: 35904391
doi: 10.1111/ina.13075
doi:

Substances chimiques

Aerosols 0
Air Pollutants 0
Particulate Matter 0
Sulfates 0
Nitric Acid 411VRN1TV4
Ammonia 7664-41-7

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

e13075

Informations de copyright

© 2022 John Wiley & Sons A/S. Published by John Wiley & Sons Ltd.

Références

Pope CA, Burnett RT, Thun MJ, et al. Lung cancer, cardiopulmonary mortality, and long-term exposure to fine particulate air pollution. JAMA. 2002;287:1132-1141.
Klepeis NE, Nelson WC, Ott WR, et al. The National Human Activity Pattern Survey (NHAPS): a resource for assessing exposure to environmental pollutants. J Expo Anal Environ Epidemiol. 2001;11:231-252.
Johnson AM, Waring MS, DeCarlo PF. Real-time transformation of outdoor aerosol components upon transport indoors measured with aerosol mass spectrometry. Indoor Air. 2017;27:230-240.
Wallace L, Williams R, Rea A, Groghan C. Erratum to “Continuous weeklong measurements of personal exposures and indoor concentrations of fine particles for 37 health-impaired North Carolina residents for up to four seasons”. Atmos Environ. 2006;40:7659-7660.
Waring MS, Siegel JA. Particle loading rates for HVAC filters, heat exchangers, and ducts. Indoor Air. 2008;18:209-224.
Chen X, Day D, Schichtel B, et al. Seasonal ambient ammonia and ammonium concentrations in a pilot IMPROVE NHx monitoring network in the western United States. Atmos Environ. 1994;2014(91):118-126.
El Orch Z, Stephens B, Waring MS. Predictions and determinants of size-resolved particle infiltration factors in single-family homes in the U.S. Build Environ. 2014;74:106-118.
Lai ACK, Thatcher TL, Nazaroff WW. Inhalation transfer factors for air pollution health risk assessment. J Air Waste Manage Assoc. 1995;2011(50):1688-1699.
Riley WJ, McKone TE, Lai ACK, Nazaroff WW. Indoor particulate matter of outdoor origin:  importance of size-dependent removal mechanisms. Environ Sci Technol. 2002;36:200-207.
Hanley JT, Ensor DS, Smith DD, Sparks LE. Fractional aerosol filtration efficiency of in-duct ventilation air cleaners. Indoor Air. 1994;4:169-178.
Cappa CD, Jimenez JL. Quantitative estimates of the volatility of ambient organic aerosol. Atmos Chem Phys. 2010;10:5409-5424.
Huffman JA, Docherty KS, Aiken AC, et al. Chemically-resolved aerosol volatility measurements from two megacity field studies. Atmos Chem Phys. 2009;9:7161-7182.
Zhang RY, Khalizov AF, Pagels J, Zhang D, Xue HX, McMurry PH. Variability in morphology, hygroscopicity, and optical properties of soot aerosols during atmospheric processing. Proc Natl Acad Sci U S A. 2008;105:10291-10296.
Avery AM, Waring MS, DeCarlo PF. Seasonal variation in aerosol composition and concentration upon transport from the outdoor to indoor environment. Environ Sci Process Impacts. 2019;21:528-547.
Liu C, Wang H, Guo H. Redistribution of PM2.5-associated nitrate and ammonium during outdoor-to-indoor transport. Indoor Air. 2019;29:460-468.
Lunden MM, Revzan KL, Fischer ML, et al. The transformation of outdoor ammonium nitrate aerosols in the indoor environment. Atmos Environ. 2003;37:5633-5644.
Sangiorgi G, Ferrero L, Ferrini BS, et al. Indoor airborne particle sources and semi-volatile partitioning effect of outdoor fine PM in offices. Atmos Environ. 2013;65:205-214.
Cummings BE, Avery AM, DeCarlo PF, Waring MS. Improving predictions of indoor aerosol concentrations of outdoor origin by considering the phase change of Semivolatile material driven by temperature and mass-loading gradients. Environ Sci Technol. 2021;55:9000-9011.
Hodas N, Turpin BJ. Shifts in the gas-particle partitioning of ambient organics with transport into the indoor environment. Aerosol Sci Technol. 2014;48:271-281.
Hering SV, Lunden MM, Thatcher TL, Kirchstetter TW, Brown NI. Using regional data and building leakage to assess indoor concentrations of particles of outdoor origin. Aerosol Sci Technol. 2007;41:639-654.
Cummings BE, Waring MS. Predicting the importance of oxidative aging on indoor organic aerosol concentrations using the two-dimensional volatility basis set (2D-VBS). Indoor Air. 2019;29:616-629.
Cummings BE, Li Y, DeCarlo PF, Shiraiwa M, Waring MS. Indoor aerosol water content and phase state in U.S. residences: impacts of relative humidity, aerosol mass and composition, and mechanical system operation. Environ Sci Process Impacts. 2020;22:2031-2057.
Shiraiwa M, Carslaw N, Tobias DJ, et al. Modelling consortium for chemistry of indoor environments (MOCCIE): integrating chemical processes from molecular to room scales. Environ Sci Process Impacts. 2019;21:1240-1254.
Donahue NM, Epstein SA, Pandis SN, Robinson AL. A two-dimensional volatility basis set: 1. Organic-aerosol mixing thermodynamics. Atmos Chem Phys. 2011;11:3303-3318.
Donahue NM, Kroll JH, Pandis SN, Robinson AL. A two-dimensional volatility basis set - part 2: diagnostics of organic-aerosol evolution. Atmos Chem Phys. 2012;12:615-634.
Jimenez JL, Canagaratna MR, Donahue NM, et al. Evolution of organic aerosols in the atmosphere. Science. 2009;326:1525-1529.
Pankow JF. An absorption model of gas/particle partitioning of organic compounds in the atmosphere. Atmos Environ. 1994;28:185-188.
Bey I, Jacob DJ, Yantosca RM, et al. Global modeling of tropospheric chemistry with assimilated meteorology: model description and evaluation. J Geophys Res-Atmos. 2001;106:23073-23095.
Byun D, Schere KL. Review of the governing equations, computational algorithms, and other components of the Models-3 community multiscale air quality (CMAQ) modeling system. Appl Mech Rev. 2006;59:51-77.
Capps SL, Henze DK, Hakami A, Russell AG, Nenes A. ANISORROPIA: the adjoint of the aerosol thermodynamic model ISORROPIA. Atmos Chem Phys. 2012;12:527-543.
Pye HOT, Liao H, Wu S, et al. Effect of changes in climate and emissions on future sulfate-nitrate-ammonium aerosol levels in the United States. J Geophys Res Atmos. 2009;114:18.
Fountoukis C, Nenes A. ISORROPIA II: A computationally efficient thermodynamic equilibrium model for K+-Ca2+-Mg2+-NH4+-Na+-SO42−-NO3−-Cl−-H2O aerosols. Atmos Chem Phys. 2007;7:4639-4659.
Nenes A, Pandis SN, Pilinis C. ISORROPIA: a new thermodynamic equilibrium model for multiphase multicomponent inorganic aerosols. Aquat Geochem. 1998;4:123-152.
Hennigan CJ, Izumi J, Sullivan AP, Weber RJ, Nenes A. A critical evaluation of proxy methods used to estimate the acidity of atmospheric particles. Atmos Chem Phys. 2015;15:2775-2790.
Song S, Gao M, Xu W, et al. Fine-particle pH for Beijing winter haze as inferred from different thermodynamic equilibrium models. Atmos Chem Phys. 2018;18:7423-7438.
Thatcher TL, Lai ACK, Moreno-Jackson R, Sextro RG, Nazaroff WW. Effects of room furnishings and air speed on particle deposition rates indoors. Atmos Environ. 2002;36:1811-1819.
Loupa G, Charpantidou E, Karageorgos E, Rapsomanikis S. The chemistry of gaseous acids in medieval churches in Cyprus. Atmos Environ. 1994;2007(41):9018-9029.
Ampollini L, Katz E, Bourne S, et al. Observations and Contributions of Real-Time Indoor Ammonia Concentrations during HOMEChem. Environ Sci Technol. 2019;53:8591-8598. doi:10.1021/acs.est.9b02157
Li M, Weschler C, Bekö G, Wargocki P, Lucic G, Williams J. Human ammonia emission rates under various indoor environmental conditions. Environ Sci Technol. 2020;54:5419-5428.
Persily A, de Jonge L. Carbon dioxide generation rates for building occupants. Indoor Air. 2017;27:868-879.
Rackes A, Waring MS. Modeling impacts of dynamic ventilation strategies on indoor air quality of offices in six US cities. Build Environ. 2013;60:243-253.
DeCarlo PF, Kimmel JR, Trimborn A, et al. Field-deployable, high-resolution, time-of-flight aerosol mass spectrometer. Anal Chem. 2006;78:8281-8289.
Pye HOT, Nenes A, Alexander B, et al. The acidity of atmospheric particles and clouds. Atmos Chem Phys Discuss. 2020;20:4809-4888.
Guo H, Sullivan AP, Campuzano-Jost P, et al. Fine particle pH and the partitioning of nitric acid during winter in the northeastern United States. J Geophys Res Atmos. 2016;121:10355-10376.
Guo H, Xu L, Bougiatioti A, et al. Fine-particle water and pH in the southeastern United States. Atmos Chem Phys. 2015;15:5211-5228.
Wild RJ, Edwards PM, Bates TS, et al. Reactive nitrogen partitioning and its relationship to winter ozone events in Utah. Atmos Chem Phys. 2016;16:573-583.
Tang YS, Braban CF, Dragosits U, et al. Acid gases and aerosol measurements in the UK(1999-2015): regional distributions and trends. Atmos Chem Phys. 2018;18:16293-16324.
DeCarlo PF, Avery AM, Waring MS. Thirdhand smoke uptake to aerosol particles in the indoor environment. Sci Adv. 2018;4:eaap8368.

Auteurs

Bryan C Berman (BC)

Department of Civil, Architectural and Environmental Engineering, Drexel University, Philadelphia, Pennsylvania, USA.

Bryan E Cummings (BE)

Department of Civil, Architectural and Environmental Engineering, Drexel University, Philadelphia, Pennsylvania, USA.

Anita M Avery (AM)

Aerodyne Research, Inc., Billerica, Massachusetts, USA.

Peter F DeCarlo (PF)

Department of Environmental Health and Engineering, Johns Hopkins University, Baltimore, Maryland, USA.

Shannon L Capps (SL)

Department of Civil, Architectural and Environmental Engineering, Drexel University, Philadelphia, Pennsylvania, USA.

Michael S Waring (MS)

Department of Civil, Architectural and Environmental Engineering, Drexel University, Philadelphia, Pennsylvania, USA.

Articles similaires

Aerosols Humans Decontamination Air Microbiology Masks
India Carbon Sequestration Environmental Monitoring Carbon Biomass
Rivers Turkey Biodiversity Environmental Monitoring Animals
1.00
Iran Environmental Monitoring Seasons Ecosystem Forests

Classifications MeSH