The first balloon-borne sample analysis of atmospheric carbonaceous components reveals new insights into formation processes.

DESI Orbitrap Organic aerosols Stratosphere Troposphere

Journal

Chemosphere
ISSN: 1879-1298
Titre abrégé: Chemosphere
Pays: England
ID NLM: 0320657

Informations de publication

Date de publication:
Jun 2023
Historique:
received: 09 11 2022
revised: 08 03 2023
accepted: 14 03 2023
medline: 5 4 2023
pubmed: 20 3 2023
entrez: 19 3 2023
Statut: ppublish

Résumé

Atmospheric aerosol optical, physical, and chemical properties play a fundamental role in the Earth's climate system. A better understanding of the processes involved in their formation, evolution, and interaction with radiation and the water cycle is critical. We report the analysis of atmospheric molecules/particles collected with a new sampling system that flew under regular weather balloons for the first time. The flight took place on January 18, 2022 from Reims (France). The samples were subsequently analyzed by high-resolution mass spectrometry (Orbitrap) to specifically infer hundreds of organic components present in 4 different layers from the troposphere to the stratosphere (up to 20 km). Additional measurements of O

Identifiants

pubmed: 36935062
pii: S0045-6535(23)00688-4
doi: 10.1016/j.chemosphere.2023.138421
pii:
doi:

Substances chimiques

Aerosols 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

138421

Informations de copyright

Copyright © 2023 Elsevier Ltd. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Roland Benoit (R)

ICARE, UPR 3021, CNRS-INSIS, Orléans, France. Electronic address: Roland.benoit@cnrs-orleans.fr.

Hazel Vernier (H)

LPC2E, UMR 7328 CNRS-Université d'Orléans-CNES, Orléans, France.

Jean-Paul Vernier (JP)

NASA Langley Research Center, Hampton, VA, USA; National Institute of Aerospace, Hampton, VA, USA.

Lilian Joly (L)

GSMA, UMR 7331 CNRS-Université de Reims Champagne-Ardenne, Reims, France.

Nicolas Dumelié (N)

GSMA, UMR 7331 CNRS-Université de Reims Champagne-Ardenne, Reims, France.

Frank G Wienhold (FG)

Federal Institute of Technology (ETHZ), Zurich, Switzerland.

Cyril Crevoisier (C)

Laboratoire de Météorologie Dynamique (LMD/IPSL), CNRS, Ecole Polytechnique, Université Paris-Saclay, Palaiseau, France.

Sandrine Delpeux (S)

ICMN, UMR 7374 CNRS-Université d'Orléans, Orléans, France.

François Bernard (F)

LPC2E, UMR 7328 CNRS-Université d'Orléans-CNES, Orléans, France.

Philippe Dagaut (P)

ICARE, UPR 3021, CNRS-INSIS, Orléans, France.

Gwenaël Berthet (G)

LPC2E, UMR 7328 CNRS-Université d'Orléans-CNES, Orléans, France.

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