Is adsorption onto activated carbon a feasible drinking water treatment option for persistent and mobile substances?

Emerging contaminants Powdered activated carbon organic micropollutants (OMP) trace organic compounds (TOrCs)

Journal

Water research
ISSN: 1879-2448
Titre abrégé: Water Res
Pays: England
ID NLM: 0105072

Informations de publication

Date de publication:
15 May 2023
Historique:
received: 28 11 2022
revised: 15 02 2023
accepted: 08 03 2023
medline: 18 4 2023
pubmed: 24 3 2023
entrez: 23 3 2023
Statut: ppublish

Résumé

Persistent and mobile (PM) substances among the organic micropollutants have gained increasing interest since their inherent properties enable them to enrich in water cycles. This study set out to investigate the potential of adsorption onto activated carbon as a drinking water treatment option for 19 PM candidates in batch experiments in a drinking water matrix using a microporous and a mesoporous activated carbon. Overall, adsorption of PM candidates proved to be very variable and the extent of removal could not be directly related to molecular properties. At an activated carbon dose of 10 mg/L and 48 h contact time, five (out of 19) substances were readily removed (≥ 80%), among them N-(3-(dimethylamino)-propyl)methacrylamide, which was investigated for the first time. For five other substances, no or negligible removal (< 20%) was observed, including 2-methyl-2-propene-1-sulfonic acid and 4‑hydroxy-1-(2-hydroxyethyl)-2,2,6,6,-tetramethylpiperidine. For the former, current state of the art adsorption processes may pose a sufficient barrier. Additionally, substance specific surrogate correlations between removals and UVA

Identifiants

pubmed: 36958222
pii: S0043-1354(23)00296-8
doi: 10.1016/j.watres.2023.119861
pii:
doi:

Substances chimiques

Charcoal 16291-96-6
Drinking Water 0
Water Pollutants, Chemical 0
isobutylene QA2LMR467H

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

119861

Informations de copyright

Copyright © 2023. Published by Elsevier Ltd.

Déclaration de conflit d'intérêts

Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Pia Schumann (P)

German Environment Agency (UBA), Section II 3.3, Schichauweg 58, 12307 Berlin, Germany; Technische Universität Berlin, Chair of Water Quality Control, Sekr. KF 4, Straße des 17. Juni 135, 10623 Berlin, Germany. Electronic address: pia.mc.schumann@campus.tu-berlin.de.

Matthias Muschket (M)

Helmholtz Centre for Environmental Research - UFZ, Permoserstraße 15, 04318 Leipzig, Germany.

Daniel Dittmann (D)

German Environment Agency (UBA), Section II 3.3, Schichauweg 58, 12307 Berlin, Germany.

Luisa Rabe (L)

German Environment Agency (UBA), Section II 3.3, Schichauweg 58, 12307 Berlin, Germany; Technische Universität Berlin, Chair of Water Quality Control, Sekr. KF 4, Straße des 17. Juni 135, 10623 Berlin, Germany.

Thorsten Reemtsma (T)

Helmholtz Centre for Environmental Research - UFZ, Permoserstraße 15, 04318 Leipzig, Germany.

Martin Jekel (M)

Technische Universität Berlin, Chair of Water Quality Control, Sekr. KF 4, Straße des 17. Juni 135, 10623 Berlin, Germany.

Aki Sebastian Ruhl (AS)

German Environment Agency (UBA), Section II 3.3, Schichauweg 58, 12307 Berlin, Germany; Technische Universität Berlin, Chair of Water Quality Control, Sekr. KF 4, Straße des 17. Juni 135, 10623 Berlin, Germany.

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Classifications MeSH