Low-dissipation self-assembly protocols of active sticky particles.


Journal

Journal of crystal growth
ISSN: 0022-0248
Titre abrégé: J Cryst Growth
Pays: Netherlands
ID NLM: 100971389

Informations de publication

Date de publication:
15 Dec 2022
Historique:
entrez: 27 3 2023
pubmed: 28 3 2023
medline: 28 3 2023
Statut: ppublish

Résumé

We use neuroevolutionary learning to identify time-dependent protocols for low-dissipation self-assembly in a model of generic active particles with interactions. When the time allotted for assembly is sufficiently long, low-dissipation protocols use only interparticle attractions, producing an amount of entropy that scales as the number of particles. When time is too short to allow assembly to proceed via diffusive motion, low-dissipation assembly protocols instead require particle self-propulsion, producing an amount of entropy that scales with the number of particles and the swim length required to cause assembly. Self-propulsion therefore provides an expensive but necessary mechanism for inducing assembly when time is of the essence.

Identifiants

pubmed: 36968622
doi: 10.1016/j.jcrysgro.2022.126912
pmc: PMC10035568
mid: NIHMS1882803
pii:
doi:

Types de publication

Journal Article

Langues

eng

Subventions

Organisme : NIGMS NIH HHS
ID : R01 GM141235
Pays : United States

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Auteurs

Stephen Whitelam (S)

Molecular Foundry, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA 94720, USA.

Jeremy D Schmit (JD)

Department of Physics, Kansas State University, Manhattan, KS, 66506, USA.

Classifications MeSH