An interlaboratory capillary zone electrophoresis-UV study of various monoclonal antibodies, instruments, and ε-aminocaproic acid lots.


Journal

Electrophoresis
ISSN: 1522-2683
Titre abrégé: Electrophoresis
Pays: Germany
ID NLM: 8204476

Informations de publication

Date de publication:
08 2023
Historique:
revised: 29 03 2023
received: 07 12 2022
accepted: 12 04 2023
medline: 17 8 2023
pubmed: 20 4 2023
entrez: 20 04 2023
Statut: ppublish

Résumé

Capillary zone electrophoresis ultraviolet (CZE-UV) has become increasingly popular for the charge heterogeneity determination of mAbs and vaccines. The ε-aminocaproic acid (eACA) CZE-UV method has been used as a rapid platform method. However, in the last years, several issues have been observed, for example, loss in electrophoretic resolution or baseline drifts. Evaluating the role of eACA on the reported issues, various laboratories were requested to provide their routinely used eACA CZE-UV methods, and background electrolyte compositions. Although every laboratory claimed to use the He et al. eACA CZE-UV method, most methods actually deviate from He's. Subsequently, a detailed interlaboratory study was designed wherein two commercially available mAbs (Waters' Mass Check Standard mAb [pI 7] and NISTmAb [pI 9]) were provided to each laboratory, along with two detailed eACA CZE-UV protocols for a short-end, high-speed, and a long-end, high-resolution method. Ten laboratories participated each using their own instruments, and commodities, showing excellence method performance (relative standard deviations [RSDs] of percent time-corrected main peak areas from 0.2% to 1.9%, and RSDs of migration times from 0.7% to 1.8% [n = 50 per laboratory], analysis times in some cases as short as 2.5 min). This study clarified that eACA is not the main reason for the abovementioned variations.

Identifiants

pubmed: 37079448
doi: 10.1002/elps.202200284
doi:

Substances chimiques

Antibodies, Monoclonal 0
Aminocaproic Acid U6F3787206
Electrolytes 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1247-1257

Informations de copyright

© 2023 The Authors. Electrophoresis published by Wiley-VCH GmbH.

Références

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Auteurs

Rebecca Wiesner (R)

Institute of Medicinal and Pharmaceutical Chemistry, Technische Universität Braunschweig, Braunschweig, Germany.

Holger Zagst (H)

Institute of Medicinal and Pharmaceutical Chemistry, Technische Universität Braunschweig, Braunschweig, Germany.

Wenkui Lan (W)

Bristol Myers Squibb, New Brunswick, New Jersey, USA.

Stewart Bigelow (S)

Health Canada, Ottawa, Ontario, Canada.

Peter Holper (P)

AB SCIEX LLC, Redwood City, California, USA.

Göran Hübner (G)

Boehringer Ingelheim Pharma GmbH & Co. KG, Biberach an der Riß, Germany.

Leila Josefsson (L)

Kantisto BV, Baarn, The Netherlands.

Claire Lancaster (C)

Regeneron Pharmaceuticals, Inc., Tarrytown, New York, USA.

Lili Lo (L)

Bristol Myers Squibb, New Brunswick, New Jersey, USA.

Christopher Lößner (C)

Boehringer Ingelheim Pharma GmbH & Co. KG, Biberach an der Riß, Germany.

Huixin Lu (H)

Health Canada, Ottawa, Ontario, Canada.

Christian Neusüß (C)

Faculty Chemistry, Hochschule Aalen, Aalen, Germany.

Carolin Rüttiger (C)

Boehringer Ingelheim Pharma GmbH & Co. KG, Biberach an der Riß, Germany.

Johannes Schlecht (J)

Faculty Chemistry, Hochschule Aalen, Aalen, Germany.

Philipp Schürrle (P)

Boehringer Ingelheim Pharma GmbH & Co. KG, Biberach an der Riß, Germany.

Alexander Selsam (A)

Boehringer Ingelheim Pharma GmbH & Co. KG, Biberach an der Riß, Germany.

Debbie van der Burg (D)

Institute of Medicinal and Pharmaceutical Chemistry, Technische Universität Braunschweig, Braunschweig, Germany.
Kantisto BV, Baarn, The Netherlands.
Department of Chemistry, School of Engineering Sciences in Chemistry, KTH Royal Institute of Technology, Stockholm, Sweden.

Shao-Chun Wang (SC)

Regeneron Pharmaceuticals, Inc., Tarrytown, New York, USA.

Yunxiao Zhu (Y)

Bristol Myers Squibb, New Brunswick, New Jersey, USA.

Hermann Wätzig (H)

Institute of Medicinal and Pharmaceutical Chemistry, Technische Universität Braunschweig, Braunschweig, Germany.

Cari Sänger-van de Griend (C)

Institute of Medicinal and Pharmaceutical Chemistry, Technische Universität Braunschweig, Braunschweig, Germany.
Kantisto BV, Baarn, The Netherlands.
Department of Medicinal Chemistry, Faculty of Pharmacy, Uppsala University, Uppsala, Sweden.

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Classifications MeSH