Microporogen-Structured Collagen Matrices for Embedded Bioprinting of Tumor Models for Immuno-Oncology.


Journal

Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358

Informations de publication

Date de publication:
Aug 2023
Historique:
revised: 10 04 2023
received: 18 11 2022
medline: 18 8 2023
pubmed: 10 5 2023
entrez: 10 5 2023
Statut: ppublish

Résumé

Embedded bioprinting enables the rapid design and fabrication of complex tissues that recapitulate in vivo microenvironments. However, few biological matrices enable good print fidelity, while simultaneously facilitate cell viability, proliferation, and migration. Here, a new microporogen-structured (µPOROS) matrix for embedded bioprinting is introduced, in which matrix rheology, printing behavior, and porosity are tailored by adding sacrificial microparticles composed of a gelatin-chitosan complex to a prepolymer collagen solution. To demonstrate its utility, a 3D tumor model is created via embedded printing of a murine melanoma cell ink within the µPOROS collagen matrix at 4 °C. The collagen matrix is subsequently crosslinked around the microparticles upon warming to 21 °C, followed by their melting and removal at 37 °C. This process results in a µPOROS matrix with a fibrillar collagen type-I network akin to that observed in vivo. Printed tumor cells remain viable and proliferate, while antigen-specific cytotoxic T cells incorporated in the matrix migrate to the tumor site, where they induce cell death. The integration of the µPOROS matrix with embedded bioprinting opens new avenues for creating complex tissue microenvironments in vitro that may find widespread use in drug discovery, disease modeling, and tissue engineering for therapeutic use.

Identifiants

pubmed: 37163476
doi: 10.1002/adma.202210748
doi:

Substances chimiques

Collagen 9007-34-5
Gelatin 9000-70-8
Hydrogels 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2210748

Subventions

Organisme : NCI NIH HHS
ID : U01CA21436901
Pays : United States

Informations de copyright

© 2023 Wiley-VCH GmbH.

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Auteurs

Daniel S Reynolds (DS)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

Irene de Lázaro (I)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

Manon L Blache (ML)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.
École Polytechnique Fédérale de Lausanne, Lausanne, 1015, Switzerland.

Yutong Liu (Y)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

Nicholas C Jeffreys (NC)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

Ramsey M Doolittle (RM)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

Estée Grandidier (E)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.
École Polytechnique Fédérale de Lausanne, Lausanne, 1015, Switzerland.
École Normale Supérieure de Lyon, Lyon, 69007, France.

Jason Olszewski (J)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.
Department of Bioengineering, Northeastern University, Boston, MA, 02115, USA.

Mason T Dacus (MT)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

David J Mooney (DJ)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

Jennifer A Lewis (JA)

John A. Paulson School of Engineering and Applied Sciences and the Wyss Institute for Biologically Inspired Engineering, Harvard University, Cambridge, MA, 02138, USA.

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