Molecular and Electronic Structures of Macrocyclic Compounds Formed at Template Synthesis in the M(II)-Thiocarbohydrazide-Diacetyl Triple Systems: A Quantum-Chemical Analysis by DFT Methods.

3,10-dithio-6,7,13,14-tetramethyl-1,2,4,5,8,9,11,12-octaazacyclotetradecatetraene-1,5,7,12 Cu(II) DFT method Ni(II) Zn(II) diacetyl template synthesis thiocarbohydrazide

Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
27 May 2023
Historique:
received: 07 05 2023
revised: 22 05 2023
accepted: 25 05 2023
medline: 12 6 2023
pubmed: 10 6 2023
entrez: 10 6 2023
Statut: epublish

Résumé

Using density functional theory (DFT) B3PW91/TZVP, M06/TZVP, and OPBE/TZVP chemistry models and the Gaussian09 program, a quantum-chemical calculation of geometric and thermodynamic parameters of Ni(II), Cu(II), and Zn(II) macrotetracyclic chelates, with (NNNN)-coordination of ligand donor centers arising during template synthesis between the indicated ions of

Identifiants

pubmed: 37298859
pii: molecules28114383
doi: 10.3390/molecules28114383
pmc: PMC10254634
pii:
doi:

Substances chimiques

thiocarbohydrazide 1IZ2H82NWU
Diacetyl K324J5K4HM
Hydrazines 0
Chelating Agents 0
Macrocyclic Compounds 0
Ligands 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Références

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Auteurs

Oleg V Mikhailov (OV)

Department of Analytical Chemistry, Certificatioin and Quality Management, Kazan National Research Technological University, K. Marx Street 68, 420015 Kazan, Russia.

Denis V Chachkov (DV)

Kazan Department of Joint Supercomputer Center of Russian Academy of Sciences-Branch of Federal Scientific Center "Scientific Research Institute for System Analysis of the RAS", Lobachevskii Street 2/31, 420111 Kazan, Russia.

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Classifications MeSH