Reduced graphene oxide/zinc oxide composite as an electrochemical sensor for acetylcholine detection.


Journal

Scientific reports
ISSN: 2045-2322
Titre abrégé: Sci Rep
Pays: England
ID NLM: 101563288

Informations de publication

Date de publication:
20 06 2024
Historique:
received: 19 02 2024
accepted: 06 06 2024
medline: 21 6 2024
pubmed: 21 6 2024
entrez: 20 6 2024
Statut: epublish

Résumé

Acetylcholine (ACh) plays a pivotal role as a neurotransmitter, influencing nerve cell communication and overall nervous system health. Imbalances in ACh levels are linked to neurodegenerative diseases, such as Alzheimer's and Parkinson's. This study focused on developing electrochemical sensors for ACh detection, utilizing graphene oxide (GO) and a composite of reduced graphene oxide and zinc oxide (rGO/ZnO). The synthesis involved modified Hummers' and hydrothermal methods, unveiling the formation of rGO through deoxygenation and the integration of nano-sized ZnO particles onto rGO, as demonstrated by XPS and TEM. EIS analysis also revealed the enhancement of electron transfer efficiency in rGO/ZnO. Cyclic voltammograms of the electrode, comprising the rGO/ZnO composite in ACh solutions, demonstrated prominent oxidation and reduction reactions. Notably, the composite exhibited promise for ACh detection due to its sensitivity, low detection threshold, reusability, and selectivity against interfering compounds, specifically glutamate and gamma-aminobutyric acid. The unique properties of rGO, such as high specific surface area and electron mobility, coupled with ZnO's stability and catalytic efficiency, contributed to the composite's potential in electrochemical sensor applications. This research, emphasizing the synthesis, fabrication, and characterization of the rGO/ZnO composite, established itself as a reliable platform for detecting the acetylcholine neurotransmitter.

Identifiants

pubmed: 38902301
doi: 10.1038/s41598-024-64238-7
pii: 10.1038/s41598-024-64238-7
doi:

Substances chimiques

Graphite 7782-42-5
Zinc Oxide SOI2LOH54Z
Acetylcholine N9YNS0M02X
graphene oxide 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

14224

Subventions

Organisme : Kasetsart University Research and Development Institute
ID : FF(KU) 25.64

Informations de copyright

© 2024. The Author(s).

Références

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Auteurs

Siraprapa Pitiphattharabun (S)

Department of Materials Engineering, Faculty of Engineering, Kasetsart University, Bangkok, Thailand.
Program of Sustainable Energy and Resources Engineering (SERE), Thailand Science Park, TAIST-Tokyo Tech, Pathumthani 12120, Thailand.

Krittin Auewattanapun (K)

Department of Materials Engineering, Faculty of Engineering, Kasetsart University, Bangkok, Thailand.

Thura Lin Htet (TL)

Department of Materials Engineering, Faculty of Engineering, Kasetsart University, Bangkok, Thailand.

Myo Myo Thu (MM)

Department of Materials Engineering, Faculty of Engineering, Kasetsart University, Bangkok, Thailand.

Gasidit Panomsuwan (G)

Department of Materials Engineering, Faculty of Engineering, Kasetsart University, Bangkok, Thailand.
International Collaborative Education Program for Materials Technology, Education, and Research (ICE-Matter), ASEAN University Network/Southeast Asia Engineering Education Development Network (AUN/SEED-Net), Bangkok, Thailand.

Ratchatee Techapiesancharoenkij (R)

Department of Materials Engineering, Faculty of Engineering, Kasetsart University, Bangkok, Thailand.
International Collaborative Education Program for Materials Technology, Education, and Research (ICE-Matter), ASEAN University Network/Southeast Asia Engineering Education Development Network (AUN/SEED-Net), Bangkok, Thailand.

Jun Ohta (J)

International Collaborative Education Program for Materials Technology, Education, and Research (ICE-Matter), ASEAN University Network/Southeast Asia Engineering Education Development Network (AUN/SEED-Net), Bangkok, Thailand.
Division of Materials Science, Nara Institute of Science and Technology, Nara, Japan.

Oratai Jongprateep (O)

Department of Materials Engineering, Faculty of Engineering, Kasetsart University, Bangkok, Thailand. fengotj@ku.ac.th.
International Collaborative Education Program for Materials Technology, Education, and Research (ICE-Matter), ASEAN University Network/Southeast Asia Engineering Education Development Network (AUN/SEED-Net), Bangkok, Thailand. fengotj@ku.ac.th.

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Humans Male Smoking Cessation Cardiovascular Diseases Female
Humans United States Aged Cross-Sectional Studies Medicare Part C
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Humans Yoga Low Back Pain Female Male

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