Formation kinetics of disinfection byproducts in algal-laden water during chlorination: A new insight into evaluating disinfection formation risk.


Journal

Environmental pollution (Barking, Essex : 1987)
ISSN: 1873-6424
Titre abrégé: Environ Pollut
Pays: England
ID NLM: 8804476

Informations de publication

Date de publication:
Feb 2019
Historique:
received: 22 06 2018
revised: 09 10 2018
accepted: 16 10 2018
pubmed: 11 11 2018
medline: 6 3 2019
entrez: 11 11 2018
Statut: ppublish

Résumé

It is necessary and important to investigate the formation of disinfection byproducts (DBPs) in water treatment systems for the management of disinfection formation risk. In the present study, the formation potential of trichloromethane (TCM) and haloacetic acids in different algal metabolites were compared, and the formation kinetics of these DBPs were investigated. The results indicated that DBP formation potential, the traditional index widely used to evaluate the disinfection formation risk, can represent neither the total precursors of DBPs nor the possible generated amounts of DBPs in drinking water systems. Kinetic analyses showed that the formation of DBPs could be well described by a classical second-order reaction kinetic model and that the actual concentrations of DBPs during chlorination were predictable with the model. The formation of DBPs in drinking water treatment systems was highly dependent on the total precursors of DBPs in water and the formation rate of DBPs with chlorine; the latter is usually underestimated in previous studies. Because of their high reactivity, TCM in hydrophilic extracellular organic matter and trichloroacetic acid in all algal metabolites should be serious considerations in the management of disinfection formation risk.

Identifiants

pubmed: 30414550
pii: S0269-7491(18)32869-0
doi: 10.1016/j.envpol.2018.10.074
pii:
doi:

Substances chimiques

Disinfectants 0
Water Pollutants, Chemical 0
Chlorine 4R7X1O2820
Trichloroacetic Acid 5V2JDO056X
Chloroform 7V31YC746X

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

63-70

Informations de copyright

Copyright © 2018 Elsevier Ltd. All rights reserved.

Auteurs

Rui Huang (R)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China.

Zhiqi Liu (Z)

Beijing Spacecrafts, Beijing, 100086, China.

Boyin Yan (B)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China.

Jingjing Zhang (J)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China.

Dongmei Liu (D)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China.

Yongpeng Xu (Y)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China.

Peng Wang (P)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China.

Fuyi Cui (F)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China; Chongqing University, Chongqing, 400044, China.

Zhiquan Liu (Z)

School of Environment, Harbin Institute of Technology, Harbin, 150090, China; Key Laboratory for Water Quality and Conservation of the Pearl River Delta, Ministry of Education, Institute of Environmental Research at Greater Bay, Guangzhou University, Guangzhou, 510006, China. Electronic address: fox_fm3@sina.com.

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Classifications MeSH