Galactosylsphingosine does not interfere with the quantitation of plasma glucosylsphingosine levels in Gaucher patients.


Journal

Clinica chimica acta; international journal of clinical chemistry
ISSN: 1873-3492
Titre abrégé: Clin Chim Acta
Pays: Netherlands
ID NLM: 1302422

Informations de publication

Date de publication:
Jul 2019
Historique:
received: 20 11 2018
revised: 14 02 2019
accepted: 07 03 2019
pubmed: 13 3 2019
medline: 14 6 2019
entrez: 13 3 2019
Statut: ppublish

Résumé

It has been shown that the plasma level of glucosylsphingosine (Lyso GL-1) is a useful biomarker for the diagnosis and monitoring of Gaucher disease. Potentially interfering with the quantitation of Lyso GL-1 is its isobaric structural isomer, galactosylsphingosine (psychosine). The contribution of psychosine is generally not accounted for in the determination of Lyso GL-1, due to the difficulty in separating these two isomers. Few methods have been presented in the literature to distinguish the two isomers, and those available tend to be tedious and time-consuming. Here, we developed a LC/MS/MS method able to chromatographically separate Lyso GL-1 and psychosine reproducibly and combine it with a simple, high-throughput sample preparation technique. We also show that the separation of these two isomers in the plasma of Gaucher patients is not necessary for the quantitation of Lyso GL-1 levels, as the relative psychosine level is <3% of Lyso GL-1.

Identifiants

pubmed: 30858093
pii: S0009-8981(19)30114-7
doi: 10.1016/j.cca.2019.03.009
pii:
doi:

Substances chimiques

Psychosine 2238-90-6
sphingosyl beta-glucoside 52050-17-6

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

48-51

Informations de copyright

Copyright © 2019 Elsevier B.V. All rights reserved.

Auteurs

Wei-Lien Chuang (WL)

Sanofi, Biomarkers and Clinical Bioanalysis, One Mountain Road, Framingham, MA 01701-9322, United States of America. Electronic address: Wei-Lien.Chuang@sanofi.com.

Joshua Pacheco (J)

Sanofi, Biomarkers and Clinical Bioanalysis, One Mountain Road, Framingham, MA 01701-9322, United States of America.

Dritan Hoxha (D)

Sanofi, Biomarkers and Clinical Bioanalysis, One Mountain Road, Framingham, MA 01701-9322, United States of America.

Gerard Sanderink (G)

Sanofi, Biomarkers and Clinical Bioanalysis, One Mountain Road, Framingham, MA 01701-9322, United States of America.

Crystal Sung (C)

Sanofi, Biomarkers and Clinical Bioanalysis, One Mountain Road, Framingham, MA 01701-9322, United States of America.

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Classifications MeSH