Experimental and numerical study of band-broadening effects associated with analyte transfer in microfluidic devices for spatial two-dimensional liquid chromatography created by additive manufacturing.

Additive manufacturing Analyte transfer Band broadening Computational fluid dynamics LC × LC Spatial chromatography

Journal

Journal of chromatography. A
ISSN: 1873-3778
Titre abrégé: J Chromatogr A
Pays: Netherlands
ID NLM: 9318488

Informations de publication

Date de publication:
02 Aug 2019
Historique:
received: 30 11 2018
revised: 19 03 2019
accepted: 20 03 2019
pubmed: 2 4 2019
medline: 30 6 2019
entrez: 2 4 2019
Statut: ppublish

Résumé

Conventional one-dimensional column-based liquid chromatographic (LC) systems do not offer sufficient separation power for the analysis of complex mixtures. Column-based comprehensive two-dimensional liquid chromatography offers a higher separation power, yet suffers from instrumental complexity and long analysis times. Spatial two-dimensional liquid chromatography can be considered as an alternative to column-based approaches. The peak capacity of the system is ideally the product of the peak capacities of the two dimensions, yet the analysis time remains relatively short due to parallel second-dimension separations. Aspects affecting the separation efficiency of this type of systems include flow distribution to homogeneously distribute the mobile phase for the second-dimension (

Identifiants

pubmed: 30929867
pii: S0021-9673(19)30309-7
doi: 10.1016/j.chroma.2019.03.041
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

77-84

Informations de copyright

Copyright © 2019 The Author(s). Published by Elsevier B.V. All rights reserved.

Auteurs

Theodora Adamopoulou (T)

Universiteit van Amsterdam, Van' t Hoff Institute for Molecular Sciences, Science Park 904, 1098 XH, Amsterdam, the Netherlands. Electronic address: t.adamopoulou@uva.nl.

Suhas Nawada (S)

Universiteit van Amsterdam, Van' t Hoff Institute for Molecular Sciences, Science Park 904, 1098 XH, Amsterdam, the Netherlands.

Sander Deridder (S)

Vrije Universiteit Brussel, Department of Chemical Engineering, Pleinlaan 2, B-1050, Brussels, Belgium.

Bert Wouters (B)

Universiteit van Amsterdam, Van' t Hoff Institute for Molecular Sciences, Science Park 904, 1098 XH, Amsterdam, the Netherlands.

Gert Desmet (G)

Vrije Universiteit Brussel, Department of Chemical Engineering, Pleinlaan 2, B-1050, Brussels, Belgium.

Peter J Schoenmakers (PJ)

Universiteit van Amsterdam, Van' t Hoff Institute for Molecular Sciences, Science Park 904, 1098 XH, Amsterdam, the Netherlands.

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Classifications MeSH