Novel SAR for quinazoline inhibitors of EHMT1 and EHMT2.


Journal

Bioorganic & medicinal chemistry letters
ISSN: 1464-3405
Titre abrégé: Bioorg Med Chem Lett
Pays: England
ID NLM: 9107377

Informations de publication

Date de publication:
01 09 2019
Historique:
received: 23 12 2018
revised: 28 05 2019
accepted: 11 06 2019
pubmed: 28 7 2019
medline: 17 9 2020
entrez: 28 7 2019
Statut: ppublish

Résumé

Detailed structure activity relationship of two series of quinazoline EHMT1/EHMT2 inhibitors (UNC0224 and UNC0638) have been elaborated. New and active alternatives are presented for the ubiquitous substitution patterns found in literature for the linker to the lysine mimicking region and the lysine mimic itself. These findings could allow for advancing EHMT1/EHMT2 inhibitors of that type beyond tool compounds by fine-tuning physicochemical properties making these inhibitors more drug-like. .

Identifiants

pubmed: 31350126
pii: S0960-894X(19)30392-0
doi: 10.1016/j.bmcl.2019.06.012
pii:
doi:

Substances chimiques

Enzyme Inhibitors 0
Histocompatibility Antigens 0
Histones 0
Quinazolines 0
EHMT1 protein, human EC 2.1.1.-
EHMT2 protein, human EC 2.1.1.43
Histone-Lysine N-Methyltransferase EC 2.1.1.43
Lysine K3Z4F929H6

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

2516-2524

Informations de copyright

Copyright © 2019 Elsevier Ltd. All rights reserved.

Auteurs

Ruben Leenders (R)

Mercachem BV, Kerkenbos 1013, 6546 BB Nijmegen, The Netherlands. Electronic address: ruben.leenders@mercachem.com.

Remco Zijlmans (R)

Mercachem BV, Kerkenbos 1013, 6546 BB Nijmegen, The Netherlands.

Bart van Bree (B)

Mercachem BV, Kerkenbos 1013, 6546 BB Nijmegen, The Netherlands.

Marc van de Sande (M)

Mercachem BV, Kerkenbos 1013, 6546 BB Nijmegen, The Netherlands.

Federica Trivarelli (F)

Mercachem BV, Kerkenbos 1013, 6546 BB Nijmegen, The Netherlands.

Eddy Damen (E)

Mercachem BV, Kerkenbos 1013, 6546 BB Nijmegen, The Netherlands.

Anita Wegert (A)

Mercachem BV, Kerkenbos 1013, 6546 BB Nijmegen, The Netherlands.

Daniel Müller (D)

ProQinase GmbH, Breisacher Strasse 117, 19106 Freiburg im Breisgau, Germany.

Jan Erik Ehlert (JE)

ProQinase GmbH, Breisacher Strasse 117, 19106 Freiburg im Breisgau, Germany.

Daniel Feger (D)

ProQinase GmbH, Breisacher Strasse 117, 19106 Freiburg im Breisgau, Germany.

Carolin Heidemann-Dinger (C)

ProQinase GmbH, Breisacher Strasse 117, 19106 Freiburg im Breisgau, Germany.

Michael Kubbutat (M)

ProQinase GmbH, Breisacher Strasse 117, 19106 Freiburg im Breisgau, Germany.

Christoph Schächtele (C)

ProQinase GmbH, Breisacher Strasse 117, 19106 Freiburg im Breisgau, Germany.

Danny C Lenstra (DC)

Radboud University, Institute for Molecules and Materials, Heyendaalseweg 135, 6525 AJ Nijmegen, The Netherlands.

Jasmin Mecinović (J)

Radboud University, Institute for Molecules and Materials, Heyendaalseweg 135, 6525 AJ Nijmegen, The Netherlands.

Gerhard Müller (G)

Gotham Therapeutics, 430 East 29th Street, New York, NY 10016, USA.

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Classifications MeSH