Selective inactivation of hypomethylating agents by SAMHD1 provides a rationale for therapeutic stratification in AML.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
02 08 2019
Historique:
received: 14 08 2018
accepted: 08 07 2019
entrez: 4 8 2019
pubmed: 4 8 2019
medline: 18 12 2019
Statut: epublish

Résumé

Hypomethylating agents decitabine and azacytidine are regarded as interchangeable in the treatment of acute myeloid leukemia (AML). However, their mechanisms of action remain incompletely understood, and predictive biomarkers for HMA efficacy are lacking. Here, we show that the bioactive metabolite decitabine triphosphate, but not azacytidine triphosphate, functions as activator and substrate of the triphosphohydrolase SAMHD1 and is subject to SAMHD1-mediated inactivation. Retrospective immunohistochemical analysis of bone marrow specimens from AML patients at diagnosis revealed that SAMHD1 expression in leukemic cells inversely correlates with clinical response to decitabine, but not to azacytidine. SAMHD1 ablation increases the antileukemic activity of decitabine in AML cell lines, primary leukemic blasts, and xenograft models. AML cells acquire resistance to decitabine partly by SAMHD1 up-regulation. Together, our data suggest that SAMHD1 is a biomarker for the stratified use of hypomethylating agents in AML patients and a potential target for the treatment of decitabine-resistant leukemia.

Identifiants

pubmed: 31375673
doi: 10.1038/s41467-019-11413-4
pii: 10.1038/s41467-019-11413-4
pmc: PMC6677770
doi:

Substances chimiques

Antimetabolites, Antineoplastic 0
Biomarkers, Tumor 0
guadecitabine 2KT4YN1DP7
Decitabine 776B62CQ27
SAM Domain and HD Domain-Containing Protein 1 EC 3.1.5.-
SAMHD1 protein, human EC 3.1.5.-
Azacitidine M801H13NRU

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

3475

Subventions

Organisme : NIAID NIH HHS
ID : R21 AI136737
Pays : United States
Organisme : NIGMS NIH HHS
ID : T32 GM008283
Pays : United States

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Auteurs

Thomas Oellerich (T)

Department of Medicine II, Hematology/Oncology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.
German Cancer Consortium/German Cancer Research Center, Heidelberg, 69120, Germany.
Frankfurt Cancer Institute, Goethe University Frankfurt, Frankfurt, 60596, Germany.

Constanze Schneider (C)

Department of Medicine II, Hematology/Oncology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.
Frankfurt Cancer Institute, Goethe University Frankfurt, Frankfurt, 60596, Germany.
Institute of Medical Virology, University of Frankfurt, Frankfurt, 60590, Germany.

Dominique Thomas (D)

pharmazentrum frankfurt/ZAFES, Institute of Clinical Pharmacology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.

Kirsten M Knecht (KM)

Department of Molecular Biophysics and Biochemistry, Yale University, New Haven, CT, 06520, USA.

Olga Buzovetsky (O)

Department of Molecular Biophysics and Biochemistry, Yale University, New Haven, CT, 06520, USA.

Lars Kaderali (L)

Institute of Bioinformatics, University Medicine Greifswald, Greifswald, 17475, Germany.

Christoph Schliemann (C)

Department of Medicine A, University Hospital Münster, Münster, 48149, Germany.

Hanibal Bohnenberger (H)

Institute of Pathology, University Medical Center, Göttingen, 37075, Germany.

Linus Angenendt (L)

Department of Medicine A, University Hospital Münster, Münster, 48149, Germany.

Wolfgang Hartmann (W)

Gerhard Domagk Institute for Pathology, University Hospital Münster, Münster, 48149, Germany.

Eva Wardelmann (E)

Gerhard Domagk Institute for Pathology, University Hospital Münster, Münster, 48149, Germany.

Tamara Rothenburger (T)

Institute of Medical Virology, University of Frankfurt, Frankfurt, 60590, Germany.

Sebastian Mohr (S)

Department of Medicine II, Hematology/Oncology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.

Sebastian Scheich (S)

Department of Medicine II, Hematology/Oncology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.

Federico Comoglio (F)

Department of Haematology, Cambridge Institute of Medical Research, Cambridge University, Cambridge, CB2 0XY, UK.

Anne Wilke (A)

Department of Medicine II, Hematology/Oncology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.

Philipp Ströbel (P)

Institute of Pathology, University Medical Center, Göttingen, 37075, Germany.

Hubert Serve (H)

Department of Medicine II, Hematology/Oncology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.
German Cancer Consortium/German Cancer Research Center, Heidelberg, 69120, Germany.
Frankfurt Cancer Institute, Goethe University Frankfurt, Frankfurt, 60596, Germany.

Martin Michaelis (M)

Industrial Biotechnology Centre and School of Biosciences, University of Kent, Canterbury, CT2 7NJ, UK.

Nerea Ferreirós (N)

pharmazentrum frankfurt/ZAFES, Institute of Clinical Pharmacology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.

Gerd Geisslinger (G)

pharmazentrum frankfurt/ZAFES, Institute of Clinical Pharmacology, Goethe University of Frankfurt, Frankfurt, 60590, Germany.
Fraunhofer Institute for Molecular Biology and Applied Ecology (IME), Project group Translational Medicine and Pharmacology (TMP), Frankfurt, 60596, Germany.

Yong Xiong (Y)

Department of Molecular Biophysics and Biochemistry, Yale University, New Haven, CT, 06520, USA.

Oliver T Keppler (OT)

Institute of Medical Virology, University of Frankfurt, Frankfurt, 60590, Germany. keppler@mvp.uni-muenchen.de.
Max von Pettenkofer Institute, Virology, Faculty of Medicine, LMU München, Munich, 80336, Germany. keppler@mvp.uni-muenchen.de.

Jindrich Cinatl (J)

Institute of Medical Virology, University of Frankfurt, Frankfurt, 60590, Germany. Cinatl@em.uni-frankfurt.de.

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Classifications MeSH