Simulation-guided enzyme discovery: A new microbial source of cellobiose 2-epimerase.


Journal

International journal of biological macromolecules
ISSN: 1879-0003
Titre abrégé: Int J Biol Macromol
Pays: Netherlands
ID NLM: 7909578

Informations de publication

Date de publication:
15 Oct 2019
Historique:
received: 29 05 2019
revised: 13 07 2019
accepted: 07 08 2019
pubmed: 12 8 2019
medline: 9 4 2020
entrez: 12 8 2019
Statut: ppublish

Résumé

Cellobiose 2-epimerase (CE) is a promising industrial enzyme that can be utilized in the dairy industry. More thermostable CEs from different microorganisms are still needed for a higher lactulose productivity. This study demonstrated the feasibility to use molecular dynamics (MD) simulation as the preliminary computational filter for thermostable enzymes screening. Sequence information of eleven uncharacterized CEs were chosen to be analyzed by MD simulations. The CE from Dictyoglomus thermophilum (Dith-CE) was determined experimentally to be one of the most thermostable CEs with the highest epimerization (160 ± 6.5 U mg

Identifiants

pubmed: 31401280
pii: S0141-8130(19)33910-8
doi: 10.1016/j.ijbiomac.2019.08.075
pmc: PMC9364981
mid: NIHMS1792786
pii:
doi:

Substances chimiques

Cellobiose 16462-44-5
Lactulose 4618-18-2
Racemases and Epimerases EC 5.1.-

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

1002-1008

Subventions

Organisme : NIGMS NIH HHS
ID : R01 GM068670
Pays : United States

Informations de copyright

Copyright © 2019 Elsevier B.V. All rights reserved.

Références

Eur Biophys J. 2011 Jul;40(7):843-56
pubmed: 21533652
Nucleic Acids Res. 2018 Mar 16;46(5):2699
pubmed: 29425356
Nucleic Acids Res. 2000 Jan 1;28(1):235-42
pubmed: 10592235
Bioresour Technol. 2012 Jan;104:668-72
pubmed: 22123300
Appl Microbiol Biotechnol. 2015 Jan;99(1):175-88
pubmed: 25431014
J Biomol Struct Dyn. 2017 Aug;35(10):2123-2135
pubmed: 27366981
Biosci Biotechnol Biochem. 2013;77(1):189-93
pubmed: 23291764
Appl Microbiol Biotechnol. 2008 Jun;79(3):433-41
pubmed: 18392616
Food Chem. 2016 Sep 15;207:60-7
pubmed: 27080880
J Agric Food Chem. 2017 Mar 29;65(12):2530-2539
pubmed: 28252294
J Dairy Sci. 2015 Oct;98(10):6767-75
pubmed: 26254523
Bioresour Technol. 2017 Jun;233:305-312
pubmed: 28285222
J Chem Theory Comput. 2016 Jun 14;12(6):2489-92
pubmed: 27123810
Curr Opin Biotechnol. 2009 Dec;20(6):616-22
pubmed: 19850467
J Biomol Struct Dyn. 2019 May;37(8):2110-2117
pubmed: 30044184
Bioresour Technol. 2013 Jan;128:809-12
pubmed: 23177735
Biosci Biotechnol Biochem. 2009 Feb;73(2):400-6
pubmed: 19202279
Appl Microbiol Biotechnol. 2011 Dec;92(6):1187-96
pubmed: 21691788
Nucleic Acids Res. 2018 Jul 2;46(W1):W296-W303
pubmed: 29788355
J Biol Chem. 2014 Feb 7;289(6):3405-15
pubmed: 24362032
Microb Cell Fact. 2017 Dec 12;16(1):224
pubmed: 29233137
Biotechnol Lett. 2012 Nov;34(11):2061-8
pubmed: 22782272
J Sci Food Agric. 2017 Aug;97(10):3095-3105
pubmed: 27873314

Auteurs

Yaqin Xiao (Y)

State Key Laboratory of Food Science and Technology, Jiangnan University, Wuxi 214122, China.

Qiuming Chen (Q)

State Key Laboratory of Food Science and Technology, Jiangnan University, Wuxi 214122, China; Department of Chemistry and Chemical Biology, Harvard University, Cambridge, MA 02138, United States.

Eugene I Shakhnovich (EI)

Department of Chemistry and Chemical Biology, Harvard University, Cambridge, MA 02138, United States. Electronic address: shakhnovich@chemistry.harvard.edu.

Wenli Zhang (W)

State Key Laboratory of Food Science and Technology, Jiangnan University, Wuxi 214122, China. Electronic address: wenlizhang@jiangnan.edu.cn.

Wanmeng Mu (W)

State Key Laboratory of Food Science and Technology, Jiangnan University, Wuxi 214122, China; International Joint Laboratory on Food Safety, Jiangnan University, Wuxi 214122, China.

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Classifications MeSH