Secondary nucleotide messenger c-di-GMP exerts a global control on natural product biosynthesis in streptomycetes.


Journal

Nucleic acids research
ISSN: 1362-4962
Titre abrégé: Nucleic Acids Res
Pays: England
ID NLM: 0411011

Informations de publication

Date de publication:
20 02 2020
Historique:
accepted: 16 01 2020
revised: 17 12 2019
received: 16 08 2019
pubmed: 21 1 2020
medline: 20 3 2020
entrez: 21 1 2020
Statut: ppublish

Résumé

Cyclic dimeric 3'-5' guanosine monophosphate, c-di-GMP, is a ubiquitous second messenger controlling diverse cellular processes in bacteria. In streptomycetes, c-di-GMP plays a crucial role in a complex morphological differentiation by modulating an activity of the pleiotropic regulator BldD. Here we report that c-di-GMP plays a key role in regulating secondary metabolite production in streptomycetes by altering the expression levels of bldD. Deletion of cdgB encoding a diguanylate cyclase in Streptomycesghanaensis reduced c-di-GMP levels and the production of the peptidoglycan glycosyltransferase inhibitor moenomycin A. In contrast to the cdgB mutant, inactivation of rmdB, encoding a phosphodiesterase for the c-di-GMP hydrolysis, positively correlated with the c-di-GMP and moenomycin A accumulation. Deletion of bldD adversely affected the synthesis of secondary metabolites in S. ghanaensis, including the production of moenomycin A. The bldD-deficient phenotype is partly mediated by an increase in expression of the pleiotropic regulatory gene wblA. Genetic and biochemical analyses demonstrate that a complex of c-di-GMP and BldD effectively represses transcription of wblA, thus preventing sporogenesis and sustaining antibiotic synthesis. These results show that manipulation of the expression of genes controlling c-di-GMP pool has the potential to improve antibiotic production as well as activate the expression of silent gene clusters.

Identifiants

pubmed: 31956908
pii: 5709707
doi: 10.1093/nar/gkz1220
pmc: PMC7026642
doi:

Substances chimiques

Bacterial Proteins 0
Biological Products 0
BldD protein, Streptomyces coelicolor 0
DNA-Binding Proteins 0
Escherichia coli Proteins 0
Nucleotides 0
Transcription Factors 0
Bambermycins 11015-37-5
moenomycin A 2RO799DN06
bis(3',5')-cyclic diguanylic acid 61093-23-0
Peptidoglycan Glycosyltransferase EC 2.4.1.129
Phosphorus-Oxygen Lyases EC 4.6.-
diguanylate cyclase EC 4.6.1.-
Cyclic GMP H2D2X058MU

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1583-1598

Informations de copyright

© The Author(s) 2020. Published by Oxford University Press on behalf of Nucleic Acids Research.

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Auteurs

Roman Makitrynskyy (R)

Pharmaceutical Biology and Biotechnology, Institute of Pharmaceutical Sciences, Albert-Ludwigs University, Freiburg 79104, Germany.

Olga Tsypik (O)

Pharmaceutical Biology and Biotechnology, Institute of Pharmaceutical Sciences, Albert-Ludwigs University, Freiburg 79104, Germany.

Desirèe Nuzzo (D)

Pharmaceutical Biology and Biotechnology, Institute of Pharmaceutical Sciences, Albert-Ludwigs University, Freiburg 79104, Germany.

Thomas Paululat (T)

Organic Chemistry, University of Siegen, Siegen 57068, Germany.

David L Zechel (DL)

Department of Chemistry, Queen's University, Kingston, Ontario K7L 3N6, Canada.

Andreas Bechthold (A)

Pharmaceutical Biology and Biotechnology, Institute of Pharmaceutical Sciences, Albert-Ludwigs University, Freiburg 79104, Germany.

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Classifications MeSH