Different Electrochemical Sensor Designs Based on Diazonium Salts and Gold Nanoparticles for Pico Molar Detection of Metals.


Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
27 Aug 2020
Historique:
received: 29 07 2020
revised: 18 08 2020
accepted: 20 08 2020
entrez: 2 9 2020
pubmed: 2 9 2020
medline: 13 3 2021
Statut: epublish

Résumé

We report a comparison of sensors' performance of different hybrid nanomaterial architectures modifying an indium tin oxide (ITO) electrode surface. Diazonium salts and gold nanoparticles (AuNPs) were used as building units to design hybrid thin films of successive layers on the ITO electrode surface. Different architectures of hybrid thin films were prepared and characterized with different techniques, such as TEM, FEG-SEM, XPS, and EIS. The prepared electrodes were used to fabricate sensors for heavy metal detection and their performances were investigated using the square wave voltammetry (SWV) method. The comparison of the obtained results shows that the deposition of AuNPs on the ITO surface, and their subsequent functionalization by diazonium salt, is the best performing architecture achieving a high sensitivity in terms of the lower detection limit of pico molar.

Identifiants

pubmed: 32867096
pii: molecules25173903
doi: 10.3390/molecules25173903
pmc: PMC7504431
pii:
doi:

Substances chimiques

Diazonium Compounds 0
Tin Compounds 0
indium tin oxide 71243-84-0
Gold 7440-57-5
Copper 789U1901C5

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : Horizon 2020 Framework Programme
ID : No 734276

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Auteurs

Zouhair Ait-Touchente (Z)

Institut de Recherche de Chimie Paris, Chimie ParisTech, PSL University-CNRS, 75005 Paris, France.

Sana Falah (S)

Institut de Recherche de Chimie Paris, Chimie ParisTech, PSL University-CNRS, 75005 Paris, France.
Faculté des Sciences de Tunis, Université El Manar, Campus Universitaire El Manar II, Tunis El Manar 2029, Tunisie.

Erika Scavetta (E)

Department of Industrial Chemistry "Toso Montanari", University of Bologna, 40136 Bologna, Italy.

Mohamed M Chehimi (MM)

CNRS, ICMPE, UMR 7182, Université Paris Est Créteil, 2-8 rue Dunant, F-94320 Thiais, France.

Rachid Touzani (R)

Laboratory of Applied Chemistry & Environment, Faculty of Science, Mohammed Premier University, Oujda 60000, Morocco.

Domenica Tonelli (D)

Department of Industrial Chemistry "Toso Montanari", University of Bologna, 40136 Bologna, Italy.

Abdelhafed Taleb (A)

Institut de Recherche de Chimie Paris, Chimie ParisTech, PSL University-CNRS, 75005 Paris, France.
Sorbonne université, 4 place Jussieu, 75231 Paris, France.

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Classifications MeSH