Structural, biosynthetic and serological cross-reactive elucidation of capsular polysaccharides from Streptococcus pneumoniae serogroup 28.


Journal

Carbohydrate polymers
ISSN: 1879-1344
Titre abrégé: Carbohydr Polym
Pays: England
ID NLM: 8307156

Informations de publication

Date de publication:
15 Feb 2021
Historique:
received: 14 08 2020
revised: 21 10 2020
accepted: 23 10 2020
entrez: 28 12 2020
pubmed: 29 12 2020
medline: 15 4 2021
Statut: ppublish

Résumé

Capsular polysaccharides (CPS) are the key virulent factors in the pathogenesis of Streptococcus pneumoniae. The previously unknown CPS structures of the pneumococcal serotype 28F and 28A were thoroughly characterized by NMR spectroscopy, chemical analysis and AF4-MALS-dRI. The following repeat unit structures were determined: -4)[α-l-Rhap-[4-P-2-Gro]]-(1-3)-α-d-Sug-[6-P-Cho]-(1-3)-β-l-Rhap-[2-OAc]-(1-4)-β-d-Glcp-(1-; 28F: Sug = Glcp, Mw: 540.5 kDa; 28A: Sug = GlcpNAc, Mw: 421.9 kDa; The correlation of CPS structures with biosynthesis showed that glycosyltransferase WciU in serotypes 28F and 28A had different sugar donor specificity toward α-d-Glcp and α-d-GlcNAcp, respectively. Furthermore, latex agglutination tests of de-OAc and de-PO

Identifiants

pubmed: 33357884
pii: S0144-8617(20)31496-X
doi: 10.1016/j.carbpol.2020.117323
pii:
doi:

Substances chimiques

Immune Sera 0
Polysaccharides, Bacterial 0
Glycosyltransferases EC 2.4.-

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

117323

Informations de copyright

Copyright © 2020 Elsevier Ltd. All rights reserved.

Auteurs

Chengxin Li (C)

Department of Chemistry, Technical University of Denmark, Kgs. Lyngby, Denmark.

Katarzyna A Duda (KA)

Junior Research Group of Allergobiochemistry, Research Center Borstel, Leibniz Lungenzentrum, Airway Research Center North (ARCN), German Center for Lung Research (DZL), Borstel, Germany.

Pernille L Elverdal (PL)

SSI Diagnostica A/S, Hilleroed, Denmark.

Ian C Skovsted (IC)

SSI Diagnostica A/S, Hilleroed, Denmark.

Christian Kjeldsen (C)

Department of Chemistry, Technical University of Denmark, Kgs. Lyngby, Denmark.

David Teze (D)

Novo Nordisk Foundation Center for Biosustainability, Technical University of Denmark, Kgs. Lyngby, Denmark.

Jens Ø Duus (JØ)

Department of Chemistry, Technical University of Denmark, Kgs. Lyngby, Denmark. Electronic address: jduus@kemi.dtu.dk.

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Classifications MeSH