Monitoring Lipophilic Toxins in Seawater Using Dispersive Liquid-Liquid Microextraction and Liquid Chromatography with Triple Quadrupole Mass Spectrometry.


Journal

Toxins
ISSN: 2072-6651
Titre abrégé: Toxins (Basel)
Pays: Switzerland
ID NLM: 101530765

Informations de publication

Date de publication:
13 01 2021
Historique:
received: 25 11 2020
revised: 07 01 2021
accepted: 09 01 2021
entrez: 16 1 2021
pubmed: 17 1 2021
medline: 22 7 2021
Statut: epublish

Résumé

The use of dispersive liquid-liquid microextraction (DLLME) is proposed for the preconcentration of thirteen lipophilic marine toxins in seawater samples. For this purpose, 0.5 mL of methanol and 440 µL of chloroform were injected into 12 mL of sample. The enriched organic phase, once evaporated and reconstituted in methanol, was analyzed by reversed-phase liquid chromatography with triple-quadrupole tandem mass spectrometry. A central composite design multivariate method was used to optimize the interrelated parameters affecting DLLME efficiency. The absence of any matrix effect in the samples allowed them to be quantified against aqueous standards. The optimized procedure was validated by recovery studies, which provided values in the 82-123% range. The detection limits varied between 0.2 and 5.7 ng L

Identifiants

pubmed: 33451113
pii: toxins13010057
doi: 10.3390/toxins13010057
pmc: PMC7828625
pii:
doi:

Substances chimiques

Marine Toxins 0
Chloroform 7V31YC746X
Methanol Y4S76JWI15

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : Fundación Séneca, Spain
ID : 19888/GERM/15
Organisme : Ministry of Science
ID : PGC2018-098363-B-100

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Auteurs

Ainhoa Oller-Ruiz (A)

Department of Analytical Chemistry, Faculty of Chemistry, Regional Campus of International Excellence "Campus Mare Nostrum", University of Murcia, E-30100 Murcia, Spain.
Department of Chemical and Environmental Engineering, Regional Campus of International Excellence "Campus Mare Nostrum", Polytechnic University of Cartagena, E-30203 Cartagena, Spain.

Natalia Campillo (N)

Department of Analytical Chemistry, Faculty of Chemistry, Regional Campus of International Excellence "Campus Mare Nostrum", University of Murcia, E-30100 Murcia, Spain.

Manuel Hernández-Córdoba (M)

Department of Analytical Chemistry, Faculty of Chemistry, Regional Campus of International Excellence "Campus Mare Nostrum", University of Murcia, E-30100 Murcia, Spain.

Javier Gilabert (J)

Department of Chemical and Environmental Engineering, Regional Campus of International Excellence "Campus Mare Nostrum", Polytechnic University of Cartagena, E-30203 Cartagena, Spain.

Pilar Viñas (P)

Department of Analytical Chemistry, Faculty of Chemistry, Regional Campus of International Excellence "Campus Mare Nostrum", University of Murcia, E-30100 Murcia, Spain.

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Classifications MeSH