Adsorption of Malachite Green and Alizarin Red S Dyes Using Fe-BTC Metal Organic Framework as Adsorbent.


Journal

International journal of molecular sciences
ISSN: 1422-0067
Titre abrégé: Int J Mol Sci
Pays: Switzerland
ID NLM: 101092791

Informations de publication

Date de publication:
14 Jan 2021
Historique:
received: 16 12 2020
revised: 08 01 2021
accepted: 10 01 2021
entrez: 20 1 2021
pubmed: 21 1 2021
medline: 13 4 2021
Statut: epublish

Résumé

Synthetic organic dyes are widely used in various industrial sectors but are also among the most harmful water pollutants. In the last decade, significant efforts have been made to develop improved materials for the removal of dyes from water, in particular, on nanostructured adsorbent materials. Metal organic frameworks (MOFs) are an attractive class of hybrid nanostructured materials with an extremely wide range of applications including adsorption. In the present work, an iron-based Fe-BTC MOF, prepared according to a rapid, aqueous-based procedure, was used as an adsorbent for the removal of alizarin red S (ARS) and malachite green (MG) dyes from water. The synthesized material was characterized in detail, while the adsorption of the dyes was monitored by UV-Vis spectroscopy. An optimal adsorption pH of 4, likely due to the establishment of favorable interactions between dyes and Fe-BTC, was found. At this pH and at a temperature of 298 K, adsorption equilibrium was reached in less than 30 min following a pseudo-second order kinetics, with k″ of 4.29 × 10

Identifiants

pubmed: 33466760
pii: ijms22020788
doi: 10.3390/ijms22020788
pmc: PMC7830139
pii:
doi:

Substances chimiques

Anthraquinones 0
Coloring Agents 0
Metal-Organic Frameworks 0
Rosaniline Dyes 0
Water Pollutants, Chemical 0
Water 059QF0KO0R
malachite green 12058M7ORO
Alizarin Red S 3F3AT0Q12H
Iron E1UOL152H7

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : Ministero dell'Istruzione, dell'Università e della Ricerca
ID : DOT1304455

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Auteurs

Giulia Rossella Delpiano (GR)

Dipartimento di Scienze Chimiche e Geologiche, Università di Cagliari, Cittadella Universitaria, S.S. 554 bivio Sestu, 09042 Monserrato (CA), Italy.

Davide Tocco (D)

Dipartimento di Scienze Chimiche e Geologiche, Università di Cagliari, Cittadella Universitaria, S.S. 554 bivio Sestu, 09042 Monserrato (CA), Italy.

Luca Medda (L)

Laboratorio NEST Scuola Normale Superiore di Pisa, 56127 Pisa, Italy.

Edmond Magner (E)

Department of Chemical Sciences, Bernal Institute, University of Limerick, Limerick V94 T9PX, Ireland.

Andrea Salis (A)

Dipartimento di Scienze Chimiche e Geologiche, Università di Cagliari, Cittadella Universitaria, S.S. 554 bivio Sestu, 09042 Monserrato (CA), Italy.
Consorzio Interuniversitario per lo Sviluppo dei Sistemi a Grande Interfase (CSGI), Unità Operativa University of Cagliari, 09042 Monserrato (CA), Italy.

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Classifications MeSH