Synthesis and Characterisation of Novel Tricyclic and Tetracyclic Furoindoles: Biological Evaluation as SAHA Enhancer against Neuroblastoma and Breast Cancer Cells.


Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
22 Sep 2021
Historique:
received: 10 08 2021
revised: 08 09 2021
accepted: 14 09 2021
entrez: 13 10 2021
pubmed: 14 10 2021
medline: 18 11 2021
Statut: epublish

Résumé

The dihydropyranoindole structures were previously identified as promising scaffolds for improving the anti-cancer activity of histone deacetylase inhibitors. This work describes the synthesis of related furoindoles and their ability to synergize with suberoylanilide hydroxamic acid (SAHA) against neuroblastoma and breast cancer cells. The nucleophilic substitution of hydroxyindole methyl esters with α-haloketones yielded the corresponding arylether ketones, which were subsequently cyclized to tricyclic and tetracyclic furoindoles. The furoindoles showed promising individual cytotoxic efficiency against breast cancer cells, as well as decent SAHA enhancement against cancer cells in select cases. Interestingly, the best IC

Identifiants

pubmed: 34641289
pii: molecules26195745
doi: 10.3390/molecules26195745
pmc: PMC8510456
pii:
doi:

Substances chimiques

Heterocyclic Compounds 0
Histone Deacetylase Inhibitors 0
Ketones 0
Vorinostat 58IFB293JI

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : National Health and Medical Research Council
ID : APP1016699

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Auteurs

Murat Bingul (M)

School of Chemistry, The University of New South Wales, Sydney, NSW 2052, Australia.
Lowy Cancer Research Centre, Children's Cancer Institute, UNSW Sydney, Sydney, NSW 2031, Australia.
School of Pharmacy, Dicle University, Diyarbakır 21280, Turkey.

Greg M Arndt (GM)

Lowy Cancer Research Centre, Children's Cancer Institute, UNSW Sydney, Sydney, NSW 2031, Australia.
ACRF Drug Discovery Centre for Childhood Cancer, Children's Cancer Institute Australia for Medical Research, Lowy Cancer Research Centre, UNSW Sydney, Sydney, NSW 2052, Australia.

Glenn M Marshall (GM)

Lowy Cancer Research Centre, Children's Cancer Institute, UNSW Sydney, Sydney, NSW 2031, Australia.
Kids Cancer Centre, Sydney Children's Hospital, Randwick, NSW 2031, Australia.

David StC Black (DS)

School of Chemistry, The University of New South Wales, Sydney, NSW 2052, Australia.

Belamy B Cheung (BB)

Lowy Cancer Research Centre, Children's Cancer Institute, UNSW Sydney, Sydney, NSW 2031, Australia.
School of Women's and Children's Health, UNSW Sydney, Sydney, NSW 2052, Australia.

Naresh Kumar (N)

School of Chemistry, The University of New South Wales, Sydney, NSW 2052, Australia.

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Classifications MeSH