3D Printed Scaffolds for Monolithic Aerogel Photocatalysts with Complex Geometries.
3D printing
TiO
2
aerogels
hydrogen production
nanoparticles
photocatalysis
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
12 2021
12 2021
Historique:
revised:
30
08
2021
received:
13
07
2021
pubmed:
19
10
2021
medline:
1
1
2022
entrez:
18
10
2021
Statut:
ppublish
Résumé
Monolithic aerogels composed of crystalline nanoparticles enable photocatalysis in three dimensions, but they suffer from low mechanical stability and it is difficult to produce them with complex geometries. Here, an approach to control the geometry of the photocatalysts to optimize their photocatalytic performance by introducing carefully designed 3D printed polymeric scaffolds into the aerogel monoliths is reported. This allows to systematically study and improve fundamental parameters in gas phase photocatalysis, such as the gas flow through and the ultraviolet light penetration into the aerogel and to customize its geometric shape to a continuous gas flow reactor. Using photocatalytic methanol reforming as a model reaction, it is shown that the optimization of these parameters leads to an increase of the hydrogen production rate by a factor of three from 400 to 1200 µmol g
Identifiants
pubmed: 34661959
doi: 10.1002/smll.202104089
doi:
Types de publication
Journal Article
Research Support, Non-U.S. Gov't
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2104089Informations de copyright
© 2021 The Authors. Small published by Wiley-VCH GmbH.
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