β-elimination of hyaluronate by red king crab hyaluronidase.


Journal

Scientific reports
ISSN: 2045-2322
Titre abrégé: Sci Rep
Pays: England
ID NLM: 101563288

Informations de publication

Date de publication:
19 11 2021
Historique:
received: 24 06 2021
accepted: 03 11 2021
entrez: 20 11 2021
pubmed: 21 11 2021
medline: 8 3 2022
Statut: epublish

Résumé

Crustacean hyaluronidases are poorly understood both in terms of their enzymatic properties and in terms of their structural features. In this work, we show that the hepatopancreas homogenate of the red king crab has a hyaluronidase activity that is an order of magnitude higher than its commercial counterpart. Zymography revealed that the molecular weight of a protein with hyalorunidase activity is 40-50 kDa. Analysis of the hepatopancreas transcriptome and results of cloning and sequencing of cDNA revealed a hyaluronidase sequence with an expected molecular weight of 42.5 kDa. Further analysis showed that hyaluronat enzymatic cleavage follows the [Formula: see text]-elimination mechanism, which is well known for bacterial hyaluronidases. The results of ion-exchange chromatography showed that the final product of hyaluronate degradation is unsaturated tetrasaccharide. Thus, we identified a new hyaluronidase of higher eukaryotes, which is not integrated into the modern classification of hyaluronidases.

Identifiants

pubmed: 34799594
doi: 10.1038/s41598-021-01890-3
pii: 10.1038/s41598-021-01890-3
pmc: PMC8604925
doi:

Substances chimiques

DNA, Complementary 0
Hyaluronic Acid 9004-61-9
Hyaluronoglucosaminidase EC 3.2.1.35

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

22600

Informations de copyright

© 2021. The Author(s).

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Auteurs

Dmitrii Sliadovskii (D)

Federal Research Center "Pushchino Scientific Center for Biological Research of the RAS", Pushchino, Russia, 142290.

Tatyana Ponomareva (T)

Federal Research Center "Pushchino Scientific Center for Biological Research of the RAS", Pushchino, Russia, 142290.

Maxim Molchanov (M)

Institute of Theoretical and Experimental Biophysics of the RAS, Pushchino, Russia, 142290.

Irina Pozdnyakova-Filatova (I)

Federal Research Center "Pushchino Scientific Center for Biological Research of the RAS", G.K. Skryabin Institute of Biochemistry and Physiology of Microorganisms, Pushchino, Russia, 142290.

Maria Timchenko (M)

Federal Research Center "Pushchino Scientific Center for Biological Research of the RAS", Pushchino, Russia, 142290.

Victor Marchenkov (V)

Institute of Protein Research RAS, Pushchino, Russia, 142290.

Oleg Gusev (O)

Regulatory Genomics Research Center, Institute of Fundamental Medicine and Biology, Kazan Federal University, Kazan, Russia, 420012.
Graduate School of Medicine, Juntendo University, Tokyo , 113-8421, Japan.

Evgeny Sogorin (E)

Federal Research Center "Pushchino Scientific Center for Biological Research of the RAS", Pushchino, Russia, 142290. evgenysogorin@gmail.com.

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Classifications MeSH