Single adsorption of diclofenac and ronidazole from aqueous solution on commercial activated carbons: effect of chemical and textural properties.
Activated carbon
Adsorption mechanism
Diclofenac
Ronidazole
Surface chemistry
Journal
Environmental science and pollution research international
ISSN: 1614-7499
Titre abrégé: Environ Sci Pollut Res Int
Pays: Germany
ID NLM: 9441769
Informations de publication
Date de publication:
Feb 2023
Feb 2023
Historique:
received:
20
06
2021
accepted:
06
11
2021
pubmed:
12
1
2022
medline:
11
3
2023
entrez:
11
1
2022
Statut:
ppublish
Résumé
The importance of the textural and physicochemical characteristics upon the adsorption capacity of the commercial activated carbons (ACs) Coconut, Wood, Merck, Darco, and Norit towards ronidazole (RNZ) and diclofenac (DCF) from water solution was investigated thoroughly in this work. At pH = 7, Coconut AC and Wood AC presented the highest adsorption capacity towards RNZ (444 mg/g) and DCF (405 mg/g). The maximum mass of RNZ adsorbed onto Coconut AC was higher in this study than those outlined previously in other works. Besides, the maximum capacity of Wood AC for adsorbing DCF was comparable to those found for other ACs. The adsorption capacity of all the ACs was increased by surface area and was favored by incrementing the acidic site concentration. The π-π stacking interactions were the predominant adsorption mechanism for the RNZ and DCF adsorption on ACs, and the acidic sites favored the adsorption capacity by activating the π-π stacking. Electrostatic interactions did not influence the adsorption of RNZ on Coconut AC, but electrostatic repulsion decreased that of DCF on Wood AC. The adsorption of DCF on Wood AC was reversible but not that of RNZ on Coconut AC. Besides, the adsorption of RNZ and DCF on the Coconut and Wood ACs was endothermic in the range of 15-25 °C.
Identifiants
pubmed: 35015236
doi: 10.1007/s11356-021-17466-7
pii: 10.1007/s11356-021-17466-7
doi:
Substances chimiques
Charcoal
16291-96-6
Ronidazole
E01R4M1063
Diclofenac
144O8QL0L1
Water
059QF0KO0R
Water Pollutants, Chemical
0
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
25193-25204Subventions
Organisme : consejo nacional de ciencia y tecnología, mexicoy telecomunicaciones
ID : Catedras program
Organisme : consejo nacional de ciencia y tecnología, mexicoy telecomunicaciones
ID : project No. 864
Organisme : universidad autónoma de san luis potosí
ID : C20-FAI-10-27.27
Informations de copyright
© 2022. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.
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