Block Copolymer Synthesis by a Sequential Addition Strategy from the Organocatalytic Group Transfer Polymerization of Methyl Methacrylate to the Ring-Opening Polymerization of Lactide.

block copolymers group transfer polymerization organic catalysis of polymerization phosphazene base ring-opening polymerization

Journal

Macromolecular rapid communications
ISSN: 1521-3927
Titre abrégé: Macromol Rapid Commun
Pays: Germany
ID NLM: 9888239

Informations de publication

Date de publication:
Oct 2022
Historique:
revised: 27 06 2022
received: 26 04 2022
pubmed: 23 7 2022
medline: 22 10 2022
entrez: 22 7 2022
Statut: ppublish

Résumé

Sequential block copolymerization involving comonomers belonging to different classes, e.g., a vinyl-type monomer and a heterocycle, is a challenging task in macromolecular chemistry, as corresponding propagating species do not interconvert easily from one to the other by crossover reactions. Here, it is first evidenced that 1-methoxy 2-methyl 1-trimethylsilyloxypropene (MTS), i.e., a silyl ketene acetal (SKA)-containing initiator, can be used in presence of the P

Identifiants

pubmed: 35868609
doi: 10.1002/marc.202200395
doi:

Substances chimiques

dilactide 95-96-5
Methylmethacrylate 196OC77688
Acetals 0
Polymethyl Methacrylate 9011-14-7
Polymers 0
ketene LEP3SM032A
Methacrylates 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2200395

Subventions

Organisme : French Ministry of Education and Research and to the Agence Nationale de la Recherche (ANR) HCO_for_LLAC
ID : 18-CE07-0018-02

Informations de copyright

© 2022 The Authors. Macromolecular Rapid Communications published by Wiley-VCH GmbH.

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Auteurs

Mohamed Samir Zaky (MS)

Laboratoire de Chimie des Polymères Organiques (LCPO), UMR 5629, Université de Bordeaux, INP-ENSCBP, 16 av. Pey Berland, Pessac Cedex, 33607, France.

Gilles Guichard (G)

Univ. Bordeaux, CNRS, CBMN, UMR 5248, Institut Européen de Chimie et Biologie, 2 rue Robert Escarpit, Pessac, F-33607, France.

Daniel Taton (D)

Laboratoire de Chimie des Polymères Organiques (LCPO), UMR 5629, Université de Bordeaux, INP-ENSCBP, 16 av. Pey Berland, Pessac Cedex, 33607, France.

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