Electrochemical Site-Selective Alkylation of Azobenzenes with (Thio)Xanthenes.

C–H functionalization alkylation azobenzenes electrochemistry thioxanthenes xanthenes

Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
04 Aug 2022
Historique:
received: 16 07 2022
revised: 31 07 2022
accepted: 02 08 2022
entrez: 12 8 2022
pubmed: 13 8 2022
medline: 16 8 2022
Statut: epublish

Résumé

Herein, we first report an electrochemical methodology for the site-selective alkylation of azobenzenes with (thio)xanthenes in the absence of any transition metal catalyst or external oxidant. A variety of groups are compatible with this electrochemical alkylation, which furnishes the products in moderate to good yields.

Identifiants

pubmed: 35956916
pii: molecules27154967
doi: 10.3390/molecules27154967
pmc: PMC9370205
pii:
doi:

Substances chimiques

Azo Compounds 0
Xanthenes 0
azobenzene F0U1H6UG5C

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : The Key Project of Provincial Natural Science Research Foundation of Anhui Universities, China
ID : KJ2020A1195
Organisme : The National Science Foundation of China
ID : 21772061
Organisme : The Open Project of State Key Laboratory of Chemistry and Molecular Engineering of Medicinal Resources
ID : CMEMR2021-B14
Organisme : the Laboratory Open Project of Huaibei Normal University
ID : 2021sykf014

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Auteurs

Qiang Zhong (Q)

Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, School of Chemistry and Materials Science, Huaibei Normal University, Huaibei 235000, China.

Hui Gao (H)

Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, School of Chemistry and Materials Science, Huaibei Normal University, Huaibei 235000, China.
Key Laboratory for Chemistry and Molecular Engineering of Medicinal Resources, School of Chemistry and Pharmaceutical Sciences, Guangxi Normal University, Guilin 541004, China.

Pei-Long Wang (PL)

Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, School of Chemistry and Materials Science, Huaibei Normal University, Huaibei 235000, China.
Information College, Huaibei Normal University, Huaibei 235000, China.

Chao Zhou (C)

Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, School of Chemistry and Materials Science, Huaibei Normal University, Huaibei 235000, China.

Tao Miao (T)

Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, School of Chemistry and Materials Science, Huaibei Normal University, Huaibei 235000, China.

Hongji Li (H)

Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, School of Chemistry and Materials Science, Huaibei Normal University, Huaibei 235000, China.

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Classifications MeSH