Process Dependent Complexity in Multicomponent Gels.
co-assembly
gels
low molecular weight gelators
self-assembly
self-sorting
Journal
Macromolecular rapid communications
ISSN: 1521-3927
Titre abrégé: Macromol Rapid Commun
Pays: Germany
ID NLM: 9888239
Informations de publication
Date de publication:
Feb 2023
Feb 2023
Historique:
revised:
20
09
2022
received:
23
08
2022
pubmed:
1
10
2022
medline:
25
2
2023
entrez:
30
9
2022
Statut:
ppublish
Résumé
Mixing low molecular weight gelators (LMWGs) can be used to combine favorable properties of the individual components within a multifunctional gel. Such multicomponent systems are complex enough in themselves but the method of combining components is not commonly considered something to influence self-assembly. Herein, two multicomponent systems comprising of a naphthalene-based dipeptide hydrogelator and one of two modified naphthalene diimides (NDIs), one of which forms gels, and the other does not, are investigated. These systems are probed, examining the structures formed and their gel properties (when preparing a solution from either a mixed powder of both components or by mixing pre-formed solutions of each component) using rheology, small angle neutron scattering (SANS), and absorbance spectroscopy. It is found that by altering the method of preparation, it is can either induce self-sorting or co-assembly within the fibers formed that underpin the gel network.
Identifiants
pubmed: 36177680
doi: 10.1002/marc.202200709
doi:
Substances chimiques
Gels
0
Dipeptides
0
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2200709Subventions
Organisme : UK Research and Innovation
Organisme : Engineering and Physical Sciences Research Council
Organisme : NSF,
ID : DMR-0520547
Informations de copyright
© 2022 The Authors. Macromolecular Rapid Communications published by Wiley-VCH GmbH.
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