Zwitterionic surface modification of polyethylene via atmospheric plasma-induced polymerization of (vinylbenzyl-)sulfobetaine and evaluation of antifouling properties.


Journal

Colloids and surfaces. B, Biointerfaces
ISSN: 1873-4367
Titre abrégé: Colloids Surf B Biointerfaces
Pays: Netherlands
ID NLM: 9315133

Informations de publication

Date de publication:
Apr 2023
Historique:
received: 18 11 2022
revised: 31 01 2023
accepted: 02 02 2023
pubmed: 10 2 2023
medline: 21 3 2023
entrez: 9 2 2023
Statut: ppublish

Résumé

Zwitterionic polymer brushes were grafted from bulk polyethylene (PE) by air plasma activation of the PE surface followed by radical polymerization of the zwitterionic styrene derivative (vinylbenzyl)sulfobetaine (VBSB). Successful formation of dense poly-(VBSB)-brush layers was confirmed by goniometry, IR spectroscopy, XPS and ToF-SIMS analysis. The resulting zwitterionic layers are about 50-100 nm thick and cause extremely low contact angles of 10° (water) on the material. Correspondingly we determined a high density of > 1.0 × 10

Identifiants

pubmed: 36758459
pii: S0927-7765(23)00073-5
doi: 10.1016/j.colsurfb.2023.113195
pii:
doi:

Substances chimiques

Polyethylene 9002-88-4
sulfobetaine 8CVU22OCJW
Polymers 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

113195

Informations de copyright

Copyright © 2023 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Nils Burmeister (N)

Universität Hamburg, Department of Chemistry, Bundesstrasse 45, 20146 Hamburg, Germany.

Christel Vollstedt (C)

Universität Hamburg, Department of Microbiology and Biotechnology, Ohnhorststrasse 18, 22609 Hamburg, Germany.

Cathrin Kröger (C)

Universität Hamburg, Department of Microbiology and Biotechnology, Ohnhorststrasse 18, 22609 Hamburg, Germany.

Timo Friedrich (T)

Universität Hamburg, Department of Chemistry, Bundesstrasse 45, 20146 Hamburg, Germany.

Nico Scharnagl (N)

Helmholtz-Zentrum Hereon GmbH, Institute of Surface Science, Max-Planck-Strasse 1, 21502 Geesthacht, Germany.

Marcus Rohnke (M)

Justus-Liebig-Universität Gießen, Institute of Physical Chemistry, Heinrich-Buff-Ring 17, 35392 Giessen, Germany.

Eilika Zorn (E)

Universität Hamburg, Department of Chemistry, Bundesstrasse 45, 20146 Hamburg, Germany.

Sebastian G Wicha (SG)

Universität Hamburg, Department of Chemistry, Bundesstrasse 45, 20146 Hamburg, Germany.

Wolfgang R Streit (WR)

Universität Hamburg, Department of Microbiology and Biotechnology, Ohnhorststrasse 18, 22609 Hamburg, Germany.

Wolfgang Maison (W)

Universität Hamburg, Department of Chemistry, Bundesstrasse 45, 20146 Hamburg, Germany. Electronic address: wolfgang.maison@uni-hamburg.de.

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Classifications MeSH