Serum organophosphate flame retardants and plasticizers in Chinese females of childbearing age: Association with serum reproductive and thyroid hormones.


Journal

Chemosphere
ISSN: 1879-1298
Titre abrégé: Chemosphere
Pays: England
ID NLM: 0320657

Informations de publication

Date de publication:
Oct 2023
Historique:
received: 08 02 2023
revised: 13 06 2023
accepted: 14 06 2023
medline: 24 7 2023
pubmed: 19 6 2023
entrez: 18 6 2023
Statut: ppublish

Résumé

Organophosphate flame retardants (OPFRs) are extensively used as flame retardants and plasticizers, but their endocrine disrupting potentials have raised concerns. However, the impacts of OPFR exposures on reproductive and thyroid hormones in females remains unclear. In this study, serum concentrations of OPFRs were investigated, and levels of reproductive and thyroid hormones, including follicle-stimulating hormone (FSH), luteinizing hormone (LH), estradiol, anti-Müllerian hormone, prolactin (PRL), testosterone (T), and thyroid stimulating hormone, were analyzed in childbearing-age females undergoing in-vitro fertilization treatment from Tianjin, a coastal city in China (n = 319). Tris (2-chloroethyl) phosphate (TCEP) was the predominant OPFR, with a median concentration of 0.33 ng/mL and a detection frequency of 96.6%. In the whole population, tris(1,3-dichloro-2-propyl) phosphate (TDCIPP) and tris(2-chloroisopropyl) phosphate (TCIPP) were positively associated with T (p < 0.05), while triethyl phosphate (TEP) was negatively associated with LH (p < 0.05) and LH/FSH (p < 0.01). Particularly, TCIPP was negatively associated with PRL in the younger subgroup (age≤30, p < 0.05). Moreover, TCIPP was negatively associated with diagnostic antral follicle counting (AFC) in the mediation analysis by a dominating direct effect (p < 0.01). In conclusion, serum levels of OPFRs were significantly associated with reproductive and thyroid hormone levels and a risk of decreased ovarian reserve in childbearing-age females, with age and body mass index being significant influencing factors.

Identifiants

pubmed: 37331665
pii: S0045-6535(23)01504-7
doi: 10.1016/j.chemosphere.2023.139237
pii:
doi:

Substances chimiques

Flame Retardants 0
Follicle Stimulating Hormone 9002-68-0
Luteinizing Hormone 9002-67-9
Organophosphates 0
Phosphates 0
Plasticizers 0
Thyroid Hormones 0
tris(chloroethyl)phosphate 32IVO568B0
Gonadal Hormones 0
Pituitary Hormones, Anterior 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

139237

Informations de copyright

Copyright © 2023 Elsevier Ltd. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Yarui Liu (Y)

College of Environmental Science and Engineering, Nankai University, 38 Tongyan Road, Jinnan District, Tianjin, 300350, China; School of Environmental Science and Engineering, Academy of Environment and Ecology, Tianjin University, 92 Weijin Road, Nankai District, Tianjin, 300072, China. Electronic address: yaruiliu_irene@126.com.

Yongcheng Li (Y)

MOE Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, 38 Tongyan Road, Jinnan District, Tianjin, 300350, China. Electronic address: liyongcheng@mail.nankai.edu.cn.

Nan Xiao (N)

Department of Center for Reproductive Medicine, Tianjin Central Hospital of Gynecology Obstetrics / Tianjin Key Laboratory of Human Development and Reproductive Regulation, 156 Nankaisanma Road, Nankai District, Tianjin, 300100, China. Electronic address: nanxiao1985@126.com.

Min Liu (M)

Department of Center for Reproductive Medicine, Tianjin Central Hospital of Gynecology Obstetrics / Tianjin Key Laboratory of Human Development and Reproductive Regulation, 156 Nankaisanma Road, Nankai District, Tianjin, 300100, China. Electronic address: liuminhaobang@163.com.

Yu Wang (Y)

MOE Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, 38 Tongyan Road, Jinnan District, Tianjin, 300350, China. Electronic address: wangyu@mail.nankai.edu.cn.

Haining Luo (H)

Department of Center for Reproductive Medicine, Tianjin Central Hospital of Gynecology Obstetrics / Tianjin Key Laboratory of Human Development and Reproductive Regulation, 156 Nankaisanma Road, Nankai District, Tianjin, 300100, China. Electronic address: luohn163@163.com.

Yiming Yao (Y)

MOE Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, 38 Tongyan Road, Jinnan District, Tianjin, 300350, China. Electronic address: yimingyao@nankai.edu.cn.

Yujie Feng (Y)

School of Environmental Science and Engineering, Academy of Environment and Ecology, Tianjin University, 92 Weijin Road, Nankai District, Tianjin, 300072, China; State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, No. 73 Huanghe Road, Nangang District, Harbin, 150090, China. Electronic address: yujief@hit.edu.cn.

Shuo Wang (S)

College of Environmental Science and Engineering, Nankai University, 38 Tongyan Road, Jinnan District, Tianjin, 300350, China; Tianjin Key Laboratory of Food Science and Health, School of Medicine, Nankai University, 94 Weijin Road, Nankai District, Tianjin, 300071, China. Electronic address: wangshuo@nankai.edu.cn.

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