A Mucin-Based Bio-Ink for 3D Printing of Objects with Anti-Biofouling Properties.


Journal

Macromolecular bioscience
ISSN: 1616-5195
Titre abrégé: Macromol Biosci
Pays: Germany
ID NLM: 101135941

Informations de publication

Date de publication:
11 2023
Historique:
revised: 10 07 2023
received: 08 05 2023
medline: 7 11 2023
pubmed: 19 7 2023
entrez: 19 7 2023
Statut: ppublish

Résumé

With its potential to revolutionize the field of personalized medicine by producing customized medical devices and constructs for tissue engineering at low costs, 3D printing has emerged as a highly promising technology. Recent advancements have sparked increasing interest in the printing of biopolymeric hydrogels. However, owing to the limited printability of those soft materials, the lack of variability in available bio-inks remains a major challenge. In this study, a novel bio-ink is developed based on functionalized mucin-a glycoprotein that exhibits a multitude of biomedically interesting properties such as immunomodulating activity and strong anti-biofouling behavior. To achieve sufficient printability of the mucin-based ink, its rheological properties are tuned by incorporating Laponite XLG as a stabilizing agent. It is shown that cured objects generated from this novel bio-ink exhibit mechanical properties partially similar to that of soft tissue, show strong anti-biofouling properties, good biocompatibility, tunable cell adhesion, and immunomodulating behavior. The presented findings suggest that this 3D printable bio-ink has a great potential for a wide range of biomedical applications, including tissue engineering, wound healing, and soft robotics.

Identifiants

pubmed: 37466113
doi: 10.1002/mabi.202300198
doi:

Substances chimiques

Mucins 0
Hydrogels 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2300198

Informations de copyright

© 2023 The Authors. Macromolecular Bioscience published by Wiley-VCH GmbH.

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Auteurs

Carolin A Rickert (CA)

TUM School of Engineering and Design, Department of Materials Engineering, Technical University of Munich, Boltzmannstr. 15, 85748, Garching b. München, Germany.
Center for Functional Protein Assemblies (CPA), Technical University of Munich, Ernst-Otto-Fischer Str. 8, 85748, Garching b. München, Germany.

Salma Mansi (S)

TUM School of Engineering and Design, Department of Mechanical Engineering, Chair of Medical Materials and Implants, Technical University of Munich, Boltzmannstr. 15, 85748, Garching b. München, Germany.
Munich Institute of Biomedical Engineering and Munich Institute of Integrated Materials, Energy and Process Engineering, Technical University of Munich, Boltzmannstr. 15, 85748, Garching, Germany.

Di Fan (D)

TUM School of Engineering and Design, Department of Materials Engineering, Technical University of Munich, Boltzmannstr. 15, 85748, Garching b. München, Germany.
Center for Functional Protein Assemblies (CPA), Technical University of Munich, Ernst-Otto-Fischer Str. 8, 85748, Garching b. München, Germany.

Petra Mela (P)

TUM School of Engineering and Design, Department of Mechanical Engineering, Chair of Medical Materials and Implants, Technical University of Munich, Boltzmannstr. 15, 85748, Garching b. München, Germany.
Munich Institute of Biomedical Engineering and Munich Institute of Integrated Materials, Energy and Process Engineering, Technical University of Munich, Boltzmannstr. 15, 85748, Garching, Germany.

Oliver Lieleg (O)

TUM School of Engineering and Design, Department of Materials Engineering, Technical University of Munich, Boltzmannstr. 15, 85748, Garching b. München, Germany.
Center for Functional Protein Assemblies (CPA), Technical University of Munich, Ernst-Otto-Fischer Str. 8, 85748, Garching b. München, Germany.

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