The case for an oxidopyrylium intermediate in the mechanism of quercetin dioxygenases.

Dioxygenation ESIPT Flavonol Oxidopyrylium Photochemistry Quercetin dioxygenase

Journal

Journal of inorganic biochemistry
ISSN: 1873-3344
Titre abrégé: J Inorg Biochem
Pays: United States
ID NLM: 7905788

Informations de publication

Date de publication:
10 2023
Historique:
received: 30 03 2023
revised: 22 06 2023
accepted: 25 07 2023
medline: 21 8 2023
pubmed: 8 8 2023
entrez: 7 8 2023
Statut: ppublish

Résumé

The quercetin dioxygenases (QDOs) are unusual metalloenzymes in that they display ring-opening dioxygenase activity with several different first-row transition metal ions which do not undergo redox changes during turnover. The QDOs are also unique in that the substrate binds as an η

Identifiants

pubmed: 37549474
pii: S0162-0134(23)00225-8
doi: 10.1016/j.jinorgbio.2023.112343
pii:
doi:

Substances chimiques

Dioxygenases EC 1.13.11.-
Quercetin 9IKM0I5T1E
Flavonols 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

112343

Informations de copyright

Copyright © 2023 Elsevier Inc. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of Competing Interest The authors declare the following financial interests/personal relationships which may be considered as potential competing interests: Patrick Farmer reports financial support and equipment, drugs, or supplies were provided by Baylor University.

Auteurs

Lasien D Rymbai (LD)

Department of Chemistry and Biochemistry, Baylor University, Waco, TX 76798, United States of America.

Kevin K Klausmeyer (KK)

Department of Chemistry and Biochemistry, Baylor University, Waco, TX 76798, United States of America.

Patrick J Farmer (PJ)

Department of Chemistry and Biochemistry, Baylor University, Waco, TX 76798, United States of America. Electronic address: Patrick_Farmer@Baylor.edu.

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Classifications MeSH